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In this paper an online method for automatically reducing complex chemical mechanisms for simulations of combustion phenomena has been developed. The method is based on the Quasi Steady State Assumption (QSSA). In contrast to previous reduction schemes where chemical species are selected only when they are in steady state throughout the whole process, the present method allows for species to be selected at each operating point separately generating an adaptive chemical kinetics. The method is used for calculations of a natural gas fueled engine operating under Homogenous Charge Compression Ignition (HCCI) conditions. We discuss criteria for selecting steady state species and the influence of these criteria on the results such as concentration profiles and temperature.

SI Engine knock is caused by autoignition in the unburnt part of the mixture (end-gas) ahead of the propagating flame. Autoignition of the end-gas occurs when the temperature and pressure exceeds a critical limit when comparatively slow reactions-releasing moderate amounts of heat-transform into ignition and rapid heat release. In this paper the difference in the heat released in the end-gas-by low temperature chemistry-between lean, rich, stochiometric, and stoichiometric mixtures diluted with cooled EGR was examined by measuring the temperature in the end-gas with Dual Broadband Rotational CARS. The measured temperature history was compared with an isentropic temperature calculated from the cylinder pressure trace. The experimentally obtained values for knock onset were compared with results from a two-zone thermodynamic model including detailed chemistry modeling of the end-gas reactions.

During development of an air assisted, direct injection combustion system, it was found that an air pulse during the late part of compression stroke significantly shortened the combustion duration and extended the lean limits of the engine. The effect of an injection of pure air through an air assist direct injector was studied with Particle Image Velocimetry, PIV. Results showed that an air pulse during the compression stroke significantly speeded up in-cylinder velocities, which also was showed in the heat release analysis. A system to use low density seeding particles was developed and is presented in the paper.

A newly developed cross flow cylinder head has been used for comparison between throttled and unthrottled operation using late intake valve closing. Pressure measurements have been used for calculations of indicated load and heat-release. Emission measurements has also been made. A model was used for estimating the amount of residual gases resulting from the different load strategies. Unthrottled operation using late intake valve closing resulted in lower pumping losses, but also in increased amounts of residual gases, using this cylinder head. This is due to the special design, with one intake valve and one exhaust valve per camshaft. Late intake valve closing was achieved by phasing one of the camshafts, resulting in late exhaust valve closing as well. With very late phasing - i.e. low load - the effective compression ratio was reduced. This, in combination with high amount of residual gases, resulted in a very unstable combustion.

Laser-induced incandescence (LII) is a sensitive diagnostic technique capable of making exhaust particulate-matter measurements during transient operating conditions. This paper presents measurements of LII signals obtained from the exhaust gas of a 1.9-L TDI diesel engine. A scanning mobility particle sizer (SMPS) is used in fixed-size mode to obtain simultaneous number concentration measurements in real-time. The transient studies presented include a cranking-start/idle/shutdown sequence, on/off cycling of EGR, and rapid load changes. The results show superior temporal response of LII compared to the SMPS. Additional advantages of LII are that exhaust dilution and cooling are not required, and that the signal amplitude is directly proportional to the carbon volume fraction and its temporal decay is related to the primary particle size.

Although there seems to be a consensus regarding the low emission potential of DME, there are still different opinions about why the low NOx emissions can be obtained without negative effects on thermal efficiency. Possible explanations are: The physical properties of DME affecting the spray and the mixture formation Different shape and duration of the heat release in combination with reduced heat losses In this paper an attempt is made to increase the knowledge of DME in relation to diesel fuel with respect to heat release and NOx formation. The emphasis has been to create injection conditions as similar as possible for both fuels. For that purpose the same injection system (CR), injection pressure (270 bar), injection timing and duration have been used for the two fuels. The only differences were the diameters of the nozzle holes, which were chosen to give the same fuel energy supply, and the physical properties of the fuels.

Laser-Rayleigh imaging has been employed to measure the relative fuel concentration in the gaseous jet region of DME sprays. The measurements were performed in an optically accessible diesel truck engine equipped with a common rail injection system. A one-hole nozzle was used to guarantee that the recorded pressure history was associated with the heat release in the imaged spray. To compensate for the low compression ratio in the modified engine the inlet air was preheated. Spray development was studied for two levels of preheating, from the start of injection to the point where all fuel was consumed. The results indicate that there is a strong correlation between the amount of unburned fuel present in the cylinder and the rate of heat release at a given time. The combustion can not be described as purely premixed or purely mixing-controlled at any time, but always has an element of both. After all fuel appears to have vanished there is still an extended period of heat release.

An experimental and computational study of the near-wall combustion in a Homogeneous Charge Compression Ignition (HCCI) engine has been conducted by applying laser based diagnostic techniques in combination with numerical modeling. Our major intent was to characterize the combustion in the velocity- and thermal boundary layers. The progress of the combustion was studied by using fuel tracer LIF, the result of which was compared with LDA measurements of the velocity boundary layer along with numerical simulations of the reacting boundary layer. Time resolved images of the PLIF signal were taken and ensemble averaged images were calculated. In the fuel tracer LIF experiments, acetone was seeded into the fuel as a tracer. It is clear from the experiments that a proper set of backgrounds and laser profiles are necessary to resolve the near-wall concentration profiles, even at a qualitative level.

An ionization sensor has been used to study the combustion process in a six-cylinder lean burn, truck-sized engine fueled with natural gas and optimized for low emissions of nitric oxides. The final goal of the investigations is to study the prospects of using the ionization sensor for finding the optimal operating position with respect to low NOx emission and stable engine operation. The results indicate that unstable combustion can be detected by analyzing the coefficient of variation (CoV) of the detector current amplitude. Close relationships between this measure and the CoV of the indicated mean effective pressure have been found during an air-fuel ratio scan with fixed ignition advance.

In this paper, a theoretical study is presented where fuel rate shaping is analyzed in combination with EGR as a method for reducing NOx formation. The analytical tools used include an empirically based model to convert fuel rate to heat release rate, and a zero dimensional multizone combustion model to calculate combustion products, local flame temperatures and NOx emissions at a given heat release rate. The multizone model, which has been presented earlier, includes flame radiation and convective heat losses. Several geometrical shapes of the fuel rate are tested for different combustion timings and EGR rates. It is found that the fuel rate giving the lowest NOx formation varies with the injection timing. In order to lower the NOx emissions at normal and advanced injection timings, the fuel rate should have a rather long duration, and start at its maximum level followed by a slow decay.

This paper reports on the development of novel time resolved spectroscopic imaging techniques for the study of spark ignition phenomena in combustion cells and an SI-engine. The techniques are based on planar laser induced fluorescence imaging (PLIF) of OH radicals, on fuel tracer PLIF, and on chemiluminescence. The techniques could be achieved at repetition rates reaching several hundreds of kilo-Hz and were cycle resolved. These techniques offer a new path along which engine related diagnostics can be undertaken, providing a wealth of information on turbulent spark ignition.

It is generally accepted that knocking combustion influences the heat transfer in SI engines. However, the effects of heat transfer on the onset of knock is still not clear due to lack of experimental data of the thermal boundary layer close to the combustion chamber wall. This paper presents measurements of the temperature in the thermal boundary layer under knocking and non-knocking conditions. The temperature was measured using dual-broadband rotational Coherent anti-Stokes Raman Spectroscopy (CARS). Simultaneous time-resolved measurements of the cylinder pressure, at three different locations, and the heat flux to the wall were carried out. Optical access to the region near the combustion chamber wall was achieved by using a horseshoe-shaped combustion chamber with windows installed in the rectangular part of the chamber. This arrangement made CARS temperature measurements close to the wall possible and results are presented in the range 0.1-5 mm from the wall.

Exhaust Gas Recirculation, EGR, is one of the most effective means of reducing NOx emissions from diesel engines and is likely to be used in order to meet future emissions standards. Exhaust gases can either be used to replace some of the air that enters the engine or can be added to the intake flow. The former case has been studied in this paper. One advantage of air replacement is that the exhaust mass flow is reduced in addition to the decreased NOx formation. The objective of this study has been to take a closer look at the factors affecting NOx emissions at different EGR rates. This is done by combining heat release analysis, based on measured pressure traces and NO formation in a multi zone combustion model. The model used is an improved version of an earlier presented model [1]. One feature in the new model is the possibility to separate the NO formation during the premixed combustion from NO formed during the diffusive combustion.

A FeCrAlloy mesh-type catalyst has been used to reduce hydrocarbons (HC) and carbon monoxide (CO) emissions from a 4-stroke HCCI engine. Significant for the HCCI engine is a high compression ratio and lean mixtures, which leads to a high efficiency, low combustion temperatures and thereby low NOx emissions, <5 pmm, but also low exhaust temperatures, around 300°C. It becomes critical to: 1. Ensure that the HCCI-combustion generates as low HC emissions as possible, this can be done by very precise control of engine inlet conditions and, if possible, compression ratio. 2. Ensure that the exhaust temperature is high enough, without loosing efficiency or producing NOx; in order to get an oxidizing catalyst to work. 3. Select proper catalyst material for the catalyst so that the exhaust temperature can be as low as possible.

In an attempt to extend the upper load limit for Homogeneous Charge Compression Ignition (HCCI), supercharging in combination with Exhaust Gas Recirculation (EGR) have been applied. Two different boost pressures were used, 1.1 bar and 1.5 bar. High EGR rates were used in order to reduce the combustion rate. The highest obtained IMEP was 16 bar. This was achieved with the higher boost pressure, at close to stoichiometric conditions and with approximately 50 % EGR. Natural gas was used as the main fuel. In the case with the higher boost pressure, iso-octane was used as pilot fuel, to improve the ignition properties of the mixture. This made it possible to use a lower compression ratio and thereby reducing the maximum cylinder pressure. The tests were performed on a single cylinder engine operated at low speed (1000 rpm). The test engine was equipped with a modified cylinder head, having a Variable Compression Ratio (VCR) mechanism.

An experimental and theoretical study of the effect of thermal barriers and catalytic coatings in a Homogeneous Charge Compression Ignition (HCCI) engine has been conducted. The main intent of the study was to investigate if a thermal barrier or catalytic coating of the wall would support the oxidation of the near-wall unburned hydrocarbons. In addition, the effect of these coatings on thermal efficiency due to changed heat transfer characteristics was investigated. The experimental setup was based on a partially coated combustion chamber. The upper part of the cylinder liner, the piston top including the top land, the valves and the cylinder head were all coated. As a thermal barrier, a coating based on plasma-sprayed Al2O3 was used. The catalytic coating was based on plasma-sprayed ZrO2 doped with Platinum. The two coatings tested were of varying thickness' of 0.15, 0.25 and 0.6 mm. The compression ratio was set to 16.75:1.

The fuel distribution in an air assist direct injection engine was measured with Planar Laser Induced Fluorescence, PLIF. The engine was fueled with isooctane and 3-pentanon was used as the fuel tracer. The optical engine was of the prolonged piston type, with a quartz ring in the upper part of the cylinder. Both the fuel injector and the spark plug were centrally located in the cylinder head. Two different pistons were examined: flat piston and bowl in piston. Results show that the differences in fuel stratification are very large for the flat piston compared to the piston with a bowl.

A method for automatic reduction of detailed reaction mechanisms using simultaneous sensitivity, reaction flow and lifetime analysis has been developed and applied to a two-zone model of an SI engine fuelled with Primary Reference Fuel (PRF). Species which are less relevant for the occurrence of autoignition in the end gas are declared redundant. They are identified and eliminated for different pre-set minimum levels of reaction flow and sensitivity. The resulting skeletal mechanism is valid in the ranges of initial and boundary values for which the analyses have been performed. A measure of species lifetime is calculated from the chemical source terms, and the species with the lifetime shorter than and mass-fraction less than specified limits are selected for removal.

The cylinder to cylinder and cycle to cycle variations were measured in a production type Volvo natural gas engine. Cylinder pressure was measured in all six cylinders. Emission measurements were performed individually after all cylinders, and commonly after the turbocharger. Measurements (ECE R49 13-mode) were performed with different spark gap and two different locations for fuel injection, one before the throttle and one before the turbocharger. Heat-release and lambda calculations show substantial cylinder to cylinder variations, due to lambda variations between the cylinders. The slow burn combustion chamber, with low turbulence, results in high cycle to cycle variations (> 100% COV imep) for some of the load cases.

A theoretical investigation is presented concerning how the heat transfer process from the gas in the combustion chamber, burned as well as the unburned gas regions, to the walls is affected by the autoignition phenomenon in SI engines. The zonal model in ref. [1] is adapted for the calculations. The radiative heat flux during the heat release period and the heat transfer in the thermal boundary layer by convection are predicted for situations when autoignition has occurred. The cylinder wall temperature is also used as a parameter in this study. The effects of engine operating parameters such as engine speed, timing of ignition, duration time of flame propagation and the fuel parameter Research Octane Number, i.e., RON, on the heat flux to the walls have been studied. The heat release is calculated for a detailed chemical kinetic model, refs. [1, 2 and 3].