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Electrical connectors and terminals are widely used in the automotive industry. It is desirable to mate the electrical connections using materials or coatings with low friction force to improve the ergonomics of the assembly process while maintaining good electrical conduction over the lifetime of the vehicle. We have previously shown that plasma-enhanced chemical vapor deposition (PECVD) of graphene on gold (Au) and silver (Ag) terminals can significantly reduce the insertion force (friction force during the terminal insertion process). However, the cost of this deposition method is rather high, and its high temperature process (> 400 oC) makes it impractical for materials with low melting temperatures. For example, tin (Sn) coating with a melting temperature of 232 oC is commonly used in electrical connectors, which cannot sustain the high temperature process. In this study, reduced graphene oxide was prepared using a low-cost solution process and applied onto metallic terminals.

Inside an automobile, hundreds of connectors and electrical terminals in various locations experience different corrosive environments. These connectors and electrical terminals need to be corrosion-proof and provide a good electrical contact for a vehicle’s lifetime. Saltwater and sulfuric acid are some of the main corrosion concerns for these electrical terminals. Currently, various thin metallic layers such as gold (Au), silver (Ag), or tin (Sn) are plated with a nickel (Ni) layer on copper alloy (Cu) terminals to ensure reliable electrical conduction during service. Graphene due to its excellent chemical stability can serve as a corrosion protective layer and prevent electrochemical oxidation of metallic terminals. In this work, effects of thin graphene layers grown by plasma-enhanced chemical vapor deposition (PECVD) on Au and Ag terminals and thin-film devices were investigated. Various mechanical, thermal/humidity, and electrical tests were performed.