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This research investigates the influences of the injection timing, injection pressure, and compression ratio on the combustion and exhaust emissions in a single cylinder 1.0 L DI diesel engine operating with ultra-high EGR. Longer ignition delays due to either advancing or retarding the injection timing reduced the smoke emissions, but advancing the injection timing has the advantages of maintaining the thermal efficiency and preventing misfiring. Smokeless combustion is realized with an intake oxygen content of only 9-10% regardless of the injection pressure. Reduction in the compression ratio is effective to reduce the in-cylinder temperature and increase the ignition delay as well as to expand the smokeless combustion range in terms of EGR and IMEP. However, the thermal efficiency deteriorates with excessively low compression ratios.

A new method to simultaneously measure temperature and concentration distributions in unsteady gas jets was established with an adaptation of the laser-induced fluorescence of iodine molecules seeded into ambient gas. Using the temperature dependence of iodine fluorescence spectra, the local temperature inside jets was determined with the ratio between the fluorescence intensities of two visualized images with different wavelengths. Jet concentrations were also determined with the images for the temperature measurements. The method was applied to an unsteady argon jet injected into hot argon-iodine ambient gases. The experimental results showed that the local temperature distribution in an unsteady gas jet were quite similar to the local concentration distributions.

Diesel combustion and emissions with four kinds of oxygenated agents as main fuels were investigated. Significant improvements in smoke, particulate matter, NOx, THC, and thermal efficiency were simultaneously realized with the oxygenates, and engine noise was also remarkably reduced for the oxygenates with higher ignitability. The improvements in the exhaust emissions and the thermal efficiency depended almost entirely on the oxygen content in the fuels regardless of the oxygenate to diesel fuel blend ratios and type of oxygenate. The unburned THC emission and odor intensity under starting condition with an oxygenate were also much lower than with conventional diesel fuel.

Soot emission from diesel engines generally increases with shorter ignition lags. However, the detailed process and mechanism of this phenomenon has not been well understood. This investigation attempts to observe and analyze the in-chamber soot formation process at various ignition lags by high-speed photography of the direct flame images and laser shadowgraphs as well as the laser light extinction. In the experiment, the separation of soot concentration from the soot-fuel mixture concentration was established by subtracting the laser light extinction intensity through a non-firing chamber from that through a firing chamber. It was found that the soot concentration in the swirl chamber reached a maximum value immediately after the start of combustion, and then decreased rapidly. With shorter ignition lags, the maximum and final soot concentrations in the chamber increased.

In a DI diesel engine, THC emissions increase significantly with lower compression ratios, a low coolant temperature, or during the transient state. During the transient after a load increase, THC emissions are increased significantly to very high concentrations from just after the start of the load increase until around the 10th cycle, then rapidly decreased until the 20th cycle, before gradually decreasing to a steady state value after 1000 cycles. In the fully-warmed steady state operation with a compression ratio of 16 and diesel fuel, THC is reasonably low, but THC increases with lower coolant temperatures or during the transient period just after increasing the load. This THC increase is due to the formation of over-lean mixture with the longer ignition delay and also due to the fuel adhering to the combustion chamber walls. A low distillation temperature fuel such as normal heptane can eliminate the THC increase.

The thermal cracking and polyaromatic hydrocarbon (PAH) formation processes of dimethyl ether (DME), ethanol, and ethane were investigated with chemical kinetics to determine the soot formation mechanism of oxygenated fuels. The modeling analyzed three processes, an isothermal constant pressure condition, a temperature rising condition under a constant pressure, and an unsteady condition approximating diesel combustion. With the same mole number of oxygen atoms, the DME rich mixtures form much carbon monoxide and methane and very little non-methane HC and PAH, in comparison with ethanol or ethane mixtures. This suggests that the existence of the C-C bond promotes the formation of PAH and soot.

The combustion characteristics in a partially premixed charge compression ignition (PCCI) engine with n-hexane were compared with ordinary diesel fuel to evaluate combustion improvements with lower distillation-temperature fuels. In the PCCI engine, a lean mixture was formed reasonably with early stage injection and the additional fuel was supplied with a second stage fuel injection after ignition. With n-hexane, thermal efficiency improved while simultaneously maintaining low NOx and smokeless combustion. A CFD analysis simulated the mixture formation processes and showed that the uniformity of the mixture with the first stage injection improves with lower distillation-temperature fuels.

The fundamental parameters related to engine combustion and performances, such as, heating value, theoretical air-fuel ratio, adiabatic flame temperature, carbon dioxide (CO2), and nitric oxide (NO) emissions, specific heat and engine thermal efficiency were investigated with computations for a wide range of oxygenated fuels. The computed results showed that almost all of the above combustion-related parameters are closely related to oxygen content in the fuels regardless of the kinds or chemical structures of oxygenated fuels. An interesting finding was that with the increase in oxygen content in the fuels NO emission decreased linearly, and the engine thermal efficiency was almost unchanged below oxygen content of 30 wt-% but gradually decreased above 30 wt-%.

Direct injection of various ignition suppressors, including water, methanol, ethanol, 1-propanol, hydrogen, and methane, was implemented to control ignition timing and expand the operating range in an HCCI engine with induced DME as the main fuel. Ultra-low NOx and smoke-less combustion was realized over a wide operating range. The reaction suppressors reduced the rate of low-temperature oxidation and consequently delayed the onset of high-temperature oxidation. Analysis of the chemical kinetics showed a reduction of OH radical in the premixed charge with the suppressors. Among the ignition suppressors, alcohols had a greater impact on OH radical reduction resulting in stronger ignition suppression. Although water injection caused a greater lowering of the temperature, which also suppressed ignition, the strong chemical effect of radical reduction with methanol injection resulted in the larger impact on suppression of oxidation reaction rates.

Light naphtha, which exhibits two-stage ignition, was induced from the intake manifold for ignition enhancement and a low ignitability fuel or water, which does not exhibit low temperature oxidation, was directly injected early in the compression stroke for ignition suppression in an HCCI engine. Their quantitative balance was flexibly controlled to optimize ignition timing according to operating condition. Ultra-low NOx and smokeless combustion without knocking or misfiring was realized over a wide operating range. Alcohols inhibit low temperature oxidation more strongly than other oxygenated or unoxygenated hydrocarbons, water, and hydrogen. Chemical kinetic modeling for methanol showed a reduction of OH radical concentration before the onset of low temperature oxidation, and this may be the main mechanism by which alcohols inhibit low temperature oxidation.

The influence of aromatic content in fuels on the soot and NOx emissions from a diesel engine was analyzed under controlled ignition lags with spark-assisted operation. Monocyclic aromatic hydrocarbons and n-hexane mixtures were used as fuels, and the aromatic content was varied from 0 to 75 v-%. The experiments showed that, at the same equivalence ratio and regardless of the molecular structure of the fuel, the soot concentration in the exhaust gas could be described by a linear-combination function with two variables representing the ignition lag and C/H atom-ratio of the fuels. For unchanged ignition lags, the soot emissions increased linearly with increased C/H atom-ratios, which are controlled by the aromatic content. The degree of increase in soot emissions with increasing C/H atom-ratio decreased with decreasing equivalence ratios. The NOx emission increased slightly with increases in the C/H atom-ratio and ignition lag.

Ultra-low NOx and smokeless operation at higher loads up to half of the rated torque is attempted with large ratios of cold EGR. NOx decreases below 6 ppm (0.05 g/(kW·h)) and soot significantly increases when first decreasing the oxygen concentration to 16% with cold EGR, but after peaking at 12-14% oxygen, soot then deceases sharply to essentially zero at 9-10% oxygen while maintaining ultra low NOx and regardless of fuel injection quantity. However, at higher loads, with the oxygen concentration below 9-10%, the air/fuel ratio has to be over-rich to exceed half of rated torque, and thermal efficiency, CO, and THC deteriorate significantly. As EGR rate increases, exhaust gas emissions and thermal efficiency vary with the intake oxygen content rather than with the excess air ratio.

Two laboratory engines, one direct, injection and one indirect injection, were operated for a range of speeds, loads, injection timings, fuels, and steady and transient conditions. Rate of combustion data were derived and analyzed using a double Wiebe's function approximation. It is shown that three of the six function parameters are constant for a wide range of conditions and that the other three can be expressed as linear functions of the amount of fuel injected during ignition lag. Engine noise, smoke, and thermal efficiency correlate with the parameters describing the amount of premixed combustion and diffusive combustion duration. These characteristics may be optimized by reducing the quantity of premixed combustion while maintaining the duration of diffusive combustion to less than 60°CA.