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Approaching engineering limits for the thermal design of battery modules requires virtual prototyping and appropriate models with respect to physical depth and computational effort. A multi-scale and multi-domain model describes the electrochemical behavior of a single battery unit cell in 1D+1D at the level of intra-cell phenomena, and it applies a 3D thermal model at module level. Both models are connected within a common vehicle simulation platform. The models are discussed with special emphasis on battery degradation such as solid electrolyte interphase layer formation, decomposition and lithium plating. The performance of the electrochemical model is assessed by discharge cycles and repeated charge/discharge simulations. The thermal module model is compared to CFD reference data and studied with respect to its grid sensitivity.

Fuel cell electric vehicles are a promising technology to create CO2- neutral mobility. Model-based development approaches are key to reduce costs and to raise efficiencies. A model on vehicle system level is discussed that balances the need of physical depth and computational performance. The vehicle model comprises the domains of mechanics, electrics, thermodynamics, cooling and controls. Detailed models of the fuel cell and battery are presented as a part of the system model. The models apply electrochemical approaches and spatial resolutions up to 3D. The models of both components are validated via 3D reference simulations showing a seamless parameter transfer between system level and CFD-based simulations. The validity of the vehicle model, including the electrochemical components, is demonstrated by simulating the Toyota Mirai vehicle. Simulation results of an NEDC are compared to measurements.

Fast charging of batteries at cold conditions faces the challenge of promoting undesired cell degradation phenomena such as lithium plating. The occurrence of lithium plating is strongly related to local surface potentials and temperatures involving the scales of the electrode surface, the unit cell and the entire module or pack. A multi-scale, multi-domain model is presented, enhancing a Newman based unit cell model with consistent models for heat generation and lithium plating and integrating this 1D+1D approach into a thermal 3D model on module level. The basic equations are presented and three different plating models from literature are discussed. The thermal model is assessed in open-loop simulations and the different plating approaches are compared in charge/discharge simulations at different operating conditions. The full multi-scale, multi-domain model is applied as a virtual sensor for model-based control of fast charging at cold conditions.