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Effects of measurement method, coolant temperature and fuel composition on soot emissions were examined by engine experiments. By reducing the pressure fluctuation in the sampling line, the measured soot emissions with better stability and reproducibility could be obtained. With lower coolant temperatures, larger soot emissions were yielded at much advanced fuel injection timings. Compared to gasoline, soot emissions with a blend fuel of normal heptane, isooctane and toluene were significantly decreased, suggesting the amounts of aromatic components (toluene or others) should be increased to obtain a representative fuel for the predictive model of particulate matter in SIDI engines.

Suppression or reduction of soot emissions is an important goal in the development of automotive engines for environmental and human health purposes. A better understanding at the molecular level of the formation process of soot particles resulting from collision and aggregation of smaller particles made of Polycyclic Aromatic Hydrocarbon (PAH) is needed. In addition to experiments, computational methods are efficient and valuable tools for this purpose. As a first step in our detailed computational chemistry study, we applied Ultra-Accelerated Molecular Dynamics (UAQCMD) and Canonical Monte-Carlo (CMC) methods to investigate the nucleation process. The UA-QCMD can calculate chemical reaction dynamics 107 times faster than conventional first principle molecular dynamics methods, while CMC can calculate equilibrium properties at various temperatures, pressures, and chemical compositions.

We developed a novel ignition method called laser breakdown-assisted long-distance discharge ignition (LBALDI) that combines laser breakdown with a discharge to realize lean combustion. The creation of laser breakdown plasma between electrodes for discharge enables discharges over longer distances than those of conventional sparkplug as inferred from laser-triggered lightning or laser-triggered gas switches. This method should help realize volumetric ignition through the creation of a long-distance discharge. Experiments on the fundamental discharge and ignition of methane/air mixtures were conducted. The optimum incident time of the laser prior to the application of a high voltage was found to reduce the sparkover voltage and markedly reduce the voltage required by LBALDI under pressurized air conditions. In the ignition experiment, LBALDI showed the fastest heat release rate at the lean flammable limit.