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Spray processes, such as primary breakup, play an important role for subsequent combustion processes and emissions formation. Accurate modeling of these spray physics is therefore key to ensure faithful representation of both the global and local characteristics of the spray. However, the governing physical mechanisms underlying primary breakup in fuel sprays are still not known. Several theories have been proposed and incorporated into different engineering models for the primary breakup of fuel sprays, with the most widely employed models following an approach based on aerodynamically-induced breakup, or more recently, based on liquid turbulence-induced breakup. However, a complete validation of these breakup models and theories is lacking since no existing measurements have yielded the joint liquid mass and drop size distribution needed to fully define the spray, especially in the near-nozzle region.

For better understanding of soot formation and oxidation processes in a biodiesel spray flame, the morphology, microstructure and sizes of soot particles directly sampled in a spray flame fuelled with soy-methyl ester were investigated using transmission electron microscopy (TEM). The soot samples were taken at different axial locations in the spray flame, 40, 50 and 70 mm from injector nozzle, which correspond to soot formation, peak, and oxidation zones, respectively. The biodiesel spray flame was generated in a constant-volume combustion chamber under a diesel-like high pressure and temperature condition (6.7 MPa, 1000K). Density, diameter of primary particles and radius of gyration of soot aggregates reached a peak at 50 mm from the injector nozzle and was lower or smaller in the formation or oxidation zones of the spray.