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One of the key challenges of the wood polymer composites (WPC) is the inadequate toughness partly due to the incompatibility of the natural fibres and PP matrix. In this work, we performed the surface modification of the natural fibre by either in-situ grafting polymerization of butyl acrylate (PBA) or adsorbing matrix-compatible cationic PBA latex on the fibre surfaces. The results indicated that the mechanical properties of the polypropylene (PP) composites containing the modified fibres, unnotched Izod impact strength in particular, have been improved significantly. The influencing factors and the mechanism of toughening process have also been preliminarily investigated.