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Lightweight metals such as Al and Mg alloys have been increasingly used for reducing mass in both structural and non-structural applications in transportation industries. Joining these lightweight materials using traditional fusion welding techniques is a critical challenge for achieving optimum mechanical performance, due to degradation of the constituent materials properties during the process. Friction stir welding (FSW), a solid-state joining technique, has emerged as a promising method for joining these lightweight materials. In particular, high joining efficiency has been achieved for FSW of various Al alloys and Mg alloys separately. Recent work on FSW of dissimilar lightweight materials also show encouraging results based on quasi-static shear performance. However, coach-peel performance of such joints has not been sufficiently examined.