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To meet 2010 emission targets, optimal SCR system performance is required. In addition, attention has to be paid to in-use compliance requirements. Closed-loop control seems an attractive option to meet the formulated goals. This study deals with the potential and limitations of closed-loop SCR control. High NOx conversion in combination with acceptable NH3 slip can be realized with an open-loop control strategy. However, closed-loop control is needed to make the SCR system robust for urea dosage inaccuracy, catalyst ageing and NOx engine-out variations. Then, the system meets conformity of production and in-use compliance norms. To demonstrate the potential of closed-loop SCR control, a NOx sensor based control strategy with cross-sensitivity compensation is compared with an adaptive surface coverage/NH3 slip control strategy and an open-loop strategy. The adaptive surface coverage/NH3 slip control strategy shows best performance over simulated ESC and ETC cycles.