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Optical imaging diagnostics of combustion are most often performed in the visible spectral band, in part because camera technology is most mature in this region, but operating in the infrared (IR) provides a number of benefits. These benefits include access to emission lines of relevant chemical species (e.g. water, carbon dioxide, and carbon monoxide) and obviation of image intensifiers (avoiding reduced spatial resolution and increased cost). High-speed IR in-cylinder imaging and image processing were used to investigate the relationships between infrared images, quantitative image-derived metrics (e.g. location of the flame centroid), and measurements made with in-cylinder pressure transducers (e.g. coefficient of variation of mean effective pressure). A 9.7-liter, inline-six, natural-gas-fueled engine was modified to enable exhaust-gas recirculation (EGR) and provide borescopic optical access to one cylinder for two high-speed infrared cameras.