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Lignocellulosic biomass consists of (hemi-) cellulose and lignin. Accordingly, an integrated biorefinery will seek to valorize both streams into higher value fuels and chemicals. To this end, this study evaluated the overall combustion performance of both cellulose- and lignin derivatives, namely the high cetane number (CN) di-n-butyl ether (DnBE) and low CN anisole, respectively. Said compounds were blended both separately and together with EN590 diesel. Experiments were conducted in a single cylinder compression ignition engine, which has been optimized for improved combustion characteristics with respect to low emission levels and at the same time high fuel efficiency. The selected operating conditions have been adopted from previous “Tailor-Made Fuels from Biomass (TMFB)” work.

The current direction for Diesel combustion system development is towards homogenization, in order to reduce particulate and NOx emissions. However, a strong increase of carbon monoxide emissions (CO) is frequently noted in combination with enhanced homogenization. Therefore, the current investigation focuses on a detailed analysis of the particulate - CO trade-off using a laser-optical and multidimensional CFD investigation of the combustion process of a swirl HSDI system. The CFD methodology involves reduced kinetics for soot formation and oxidation and a three-step CO model. These models are validated by a detailed comparison to optical measurements of flow, spray penetration and the spatial distribution of soot, temperature and oxygen concentration. The results obtained show that high concentrations of CO occur as an intermediate combustion reaction product. Subsequently, CO and soot are oxidized in large areas of the combustion chamber.