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The study of vehicle coupling state estimation accuracy especially in observer-based vehicle chassis control for improving road handling and ride comfort is a challenging task for vehicle industry under various driving conditions. Due to a large amount of life safety arising from vehicle roll behavior, how to precisely acquire vehicle roll state and rapidly provide for the vehicle control system are of great concern. Simultaneously, uncertainty is unavoidable for various aspects of a vehicle system, e.g., varying sprung mass, moment of inertia and position of the center of gravity. To deal with the above issues, a novel dual observer approach, which combines adaptive Unscented Kalman Filter (AUKF) and Takagi-Sugeno (T-S), is proposed in this paper. A full-car nonlinear model is first established to describe vehicle lateral and vertical coupling roll behavior under various road excitation.