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Long chain alcohols possess major advantages over the currently used ethanol as bio-components for gasoline, including higher energy content, better engine compatibility, and less water solubility. The rapid developments in biofuel technology have made it possible to produce C 4 -C 5 alcohols cost effectively. These higher alcohols could significantly expand the biofuel content and potentially substitute ethanol in future gasoline mixtures. This study characterizes some fundamental properties of a C 5 alcohol, isopentanol, as a fuel for HCCI engines. Wide ranges of engine speed, intake temperature, intake pressure, and equivalence ratio are investigated. Results are presented in comparison with gasoline or ethanol data previously reported. For a given combustion phasing, isopentanol requires lower intake temperatures than gasoline or ethanol at all tested speeds, indicating a higher HCCI reactivity.

The potential of boosted HCCI for achieving high loads has been investigated for intake pressures (Piⁿ) from 100 kPa (naturally aspirated) to 325 kPa absolute. Experiments were conducted in a single-cylinder HCCI research engine (0.98 liters) equipped with a compression-ratio 14 piston at 1200 rpm. The intake charge was fully premixed well upstream of the intake, and the fuel was a research-grade (R+M)/2 = 87-octane gasoline with a composition typical of commercial gasolines. Beginning with Piⁿ = 100 kPa, the intake pressure was systematically increased in steps of 20 - 40 kPa, and for each Piⁿ, the fueling was incrementally increased up to the knock/stability limit, beyond which slight changes in combustion conditions can lead to strong knocking or misfire. A combination of reduced intake temperature and cooled EGR was used to compensate for the pressure-induced enhancement of autoignition and to provide sufficient combustion-phasing retard to control knock.

This work explores the high-load limits of HCCI for naturally aspirated operation. This is done for three fuels with various autoignition reactivity: iso-octane, PRF80, and PRF60. The experiments were conducted in a single-cylinder HCCI research engine (0.98 liter displacement), mostly with a CR = 14 piston installed, but with some tests at CR = 18. Five load-limiting factors were identified: 1) NOx-induced combustion-phasing run-away, 2) wall-heating-induced run-away, 3) EGR-induced oxygen deprivation, 4) wandering unsteady combustion, and 5) excessive exhaust NOx. These experiments at 1200 rpm show that the actual load-limiting factor is dependent on the autoignition reactivity of the fuel, the selected CA50, and in some cases, the tolerable level of NOx emissions. For iso-octane, which has the highest resistance to autoignition of the fuels tested, the NOx emissions become unacceptable at IMEPg = 473 kPa.

This study investigates the potential of partial fuel stratification for reducing the knocking propensity of intake-boosted HCCI engines operating on conventional gasoline. Although intake boosting can substantially increase the high-load capability of HCCI, these engines would be more production-viable if the knock/stability load limit could be extended to allow higher loads at a given boost and/or to provide even higher thermal efficiencies. A technique termed partial fuel stratification (PFS) has recently been shown to greatly reduce the combustion-induced pressure-rise rate (PRR), and therefore the knocking propensity of naturally aspirated HCCI, when the engine is fueled with a φ-sensitive, two-stage-ignition fuel. The current work explores the potential of applying PFS to boosted HCCI operation using conventional gasoline, which does not typically show two-stage ignition. Experiments were conducted in a single-cylinder HCCI research engine (0.98 liters) at 1200 rpm.

A tracer-based single-line PLIF imaging technique using a unique optical configuration that allows simultaneously viewing the bulk-gas and the boundary layer region has been applied to an investigation of the naturally occurring thermal stratification in a HCCI engine. Thermal stratification is critical for HCCI engines, because it determines the maximum pressure rise rate which is a limiting factor for high-load operation. The investigation is based on the analysis of temperature maps that were derived from PLIF images, using the temperature sensitivity of fluorescence from toluene introduced as tracer in the fuel. Measurements were made in a single-cylinder optically accessible HCCI engine operating under motored conditions with a vertical laser-sheet orientation that allows observation of the development of thermal stratification from the cold boundary layers into the central region of the charge.

Ethanol and ethanol/gasoline blends are being widely considered as alternative fuels for light-duty automotive applications. At the same time, HCCI combustion has the potential to provide high efficiency and ultra-low exhaust emissions. However, the application of HCCI is typically limited to low and moderate loads because of unacceptably high heat-release rates (HRR) at higher fueling rates. This work investigates the potential of lowering the HCCI HRR at high loads by using partial fuel stratification to increase the in-cylinder thermal stratification. This strategy is based on ethanol's high heat of vaporization combined with its true single-stage ignition characteristics. Using partial fuel stratification, the strong fuel-vaporization cooling produces thermal stratification due to variations in the amount of fuel vaporization in different parts of the combustion chamber.

Fuel stratification has been investigated as a means of improving the low-load combustion efficiency in an HCCI engine. Several stratification techniques were examined: different GDI injectors, increased swirl, and changes in injection pressure, to determine which parameters are effective for improving the combustion efficiency while maintaining NOx emissions below U.S. 2010 limits. Performance and emission measurements were obtained in an all-metal engine. Corresponding fuel distribution measurements were made with fuel PLIF imaging in a matching optically accessible engine. The fuel used was iso-octane, which is a good surrogate for gasoline. For an idle fueling rate (ϕ = 0.12), combustion efficiency was improved substantially, from 64% to 89% at the NOx limit, using delayed fuel injection with a hollow-cone injector at an injection pressure of 120 bar.

Multi-zone CFD simulations with detailed kinetics were used to model iso-octane HCCI experiments performed on a single-cylinder research engine. The modeling goals were to validate the method (multi-zone combustion modeling) and the reaction mechanism (LLNL 857 species iso-octane) by comparing model results to detailed exhaust speciation data, which was obtained with gas chromatography. The model is compared to experiments run at 1200 RPM and 1.35 bar boost pressure over an equivalence ratio range from 0.08 to 0.28. Fuel was introduced far upstream to ensure fuel and air homogeneity prior to entering the 13.8:1 compression ratio, shallow-bowl combustion chamber of this 4-stroke engine. The CFD grid incorporated a very detailed representation of the crevices, including the top-land ring crevice and head-gasket crevice. The ring crevice is resolved all the way into the ring pocket volume. The detailed grid was required to capture regions where emission species are formed and retained.

The combustion process in diesel engines deposits soot on the in-cylinder surfaces. Previous works have suggested that these soot deposits eventually break off during cylinder blow-down and the exhaust stroke and contribute significantly to exhaust soot emissions. In order to better understand this potential pathway to soot emissions, the authors recently investigated combusting fuel-jet/wall interactions in a diesel engine. This work, published as a companion paper, showed how soot escaped from the combusting fuel jet and was brought in close proximity to the wall so that it could become a deposit. The current study extends this earlier work with laser-extinction measurements of the soot-deposition rate in the same single-cylinder, heavy-duty DI diesel engine. Measurements were made by passing the beam of a CW-diode laser through a window in the piston bowl rim that was in-line with one of the fuel jets.

Over the past decade, laser diagnostics have improved our understanding of many aspects of diesel combustion. However, interactions between the combusting fuel jet and the piston-bowl wall are not well understood. In heavy-duty diesel engines, with typical fuels, these interactions occur with the combusting vapor-phase region of the jet, which consists of a central region containing soot and other products of rich-premixed combustion, surrounded by a diffusion flame. Since previous work has shown that the OH radical is a good marker of the diffusion flame, planar laser-induced fluorescence (PLIF) imaging of OH was applied to an investigation of the diffusion flame during wall interaction. In addition, simultaneous OH PLIF and planar laser-induced incandescence (PLII) soot imaging was applied to investigate the likelihood for soot deposition on the bowl wall.

To better understand the factors affecting soot formation in diesel engines, in-cylinder soot and diffusion flame lift-off were measured in a heavy-duty, direct-injection diesel engine. Measurements were obtained at two operating conditions using two commercial diesel fuels and a range of oxygenated paraffinic fuel blends. A line-of-sight laser extinction diagnostic was improved and employed to measure the relative soot concentration within the jet (“jet-soot”) and the rates of soot-wall deposition on the piston bowl-rim. An OH chemiluminescence imaging technique was developed to determine the location of the diffusion flame and to measure the lift-off lengths of the diffusion flame to estimate the amount of oxygen entrainment in the diesel jets. Both the jet-soot and the rate of soot-wall deposition were found to decrease with increasing fuel oxygen-to-carbon ratio (O/C) over a wide range of O/C.

Chemiluminescence imaging has been applied to investigate the naturally occurring charge stratification in an HCCI engine. This stratification slows the pressure-rise rate (PRR) during combustion, making it critical to the high-load operating limit of these engines. Experiments were conducted in a single-cylinder HCCI engine modified with windows in the combustion chamber for optical access. Using this engine, chemiluminescence images were obtained from three different view angles. These included both single-shot images with intensified CCD cameras and high-speed (20kHz) sequences with an intensified CMOS video camera. The engine was fueled with iso-octane, which has been shown to be a reasonable surrogate for gasoline and exhibits only single-stage ignition at these naturally aspirated conditions. The chemiluminescence images show that the HCCI combustion is not homogeneous but has a strong turbulent structure even when the fuel and air are fully premixed prior to intake.

Two methods for mitigating unacceptably high HCCI heat-release rates are investigated and compared in this combined experimental/CFD work. Retarding the combustion phasing by decreasing the intake temperature is found to have good potential for smoothing heat-release rates and reducing engine knock. There are at least three reasons for this: 1) lower combustion temperatures, 2) less pressure rise when the combustion is occurring during the expansion stroke, and 3) the natural thermal stratification increases around TDC. However, overly retarded combustion leads to unstable operation with partial-burn cycles resulting in high IMEPg variations and increased emissions. Enhanced natural thermal stratification by increased heat-transfer rates was explored by lowering the coolant temperature from 100 to 50°C. This strategy substantially decreased the heat-release rates and lowered the knocking intensity under certain conditions.

The effects of injection timing and diluent addition on the late-combustion soot burnout in a direct-injection (DI) diesel engine have been investigated using simultaneous planar imaging of the OH-radical and soot distributions. Measurements were made in an optically accessible DI diesel engine of the heavy-duty size class at a 1680 rpm, high-load operating condition. A dual-laser, dual-camera system was used to obtain the simultaneous “single-shot” images using planar laser-induced fluorescence (PLIF) and planar laser-induced incandescence (PLII) for the OH and soot, respectively. The two laser beams were combined into overlapping laser sheets before being directed into the combustion chamber, and the optical signal was separated into the two cameras by means of an edge filter.