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An engine exhaust manifold undergoes repeated thermal expansion and contraction due to temperature variation. Thermomechanical fatigue (TMF) arises due to the boundary constraints on thermal expansion so that mechanical strain is introduced. Therefore, TMF evaluation is very important in engine design. In this work, the mechanical properties important for TMF assessment and modeling of a silicon (Si)- and molybdenum (Mo)-containing ductile cast iron used for exhaust manifold have been evaluated. Tensile, creep, isothermal low cycle fatigue (LCF), and TMF tests have been conducted. Parameters for material modeling, such as the viscoplastic constitutive model and the Neu-Sehitoglu TMF damage model, have been calibrated, validated, and used to evaluate the TMF life of the exhaust manifold.