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The objective of this research is a detailed investigation of unburned hydrocarbon (UHC) in a highly-dilute diesel low temperature combustion (LTC) regime. This research concentrates on understanding the mechanisms that control the formation of UHC via experiments and simulations in a 0.48L signal-cylinder light duty engine operating at 2000 r/min and 5.5 bar IMEP with multiple injections. A multi-gas FTIR along with other gas and smoke emissions instruments are used to measure exhaust UHC species and other emissions. Controlled experiments in the single-cylinder engine are then combined with three computational tools, namely heat release analysis of measured cylinder pressure, analysis of spray trajectory with a phenomenological spray model using in-cylinder thermodynamics [1], and KIVA-3V Chemkin CFD computations recently tested at LTC conditions [2].

Negative valve overlap (NVO) is a viable control strategy that enables low-temperature gasoline combustion (LTGC) at low loads. Thermal effects of NVO fueling on main combustion are well understood, but fuel reforming chemistry during NVO has not been extensively studied. The objective of this work is to analyze the impact of global equivalence ratio and available oxidizer on NVO product concentrations. Experiments were performed in a LTGC single-cylinder engine under a sweep of NVO oxygen concentration and NVO fueling rates. Gas sampling at the start and end of the NVO period was performed via a custom dump-valve apparatus with detailed sample speciation by gas chromatography. Single-zone reactor models using detailed chemistry at relevant mixing and thermodynamic conditions were used in parallel to the experiments to evaluate expected yields of partially oxidized species under representative engine time scales.

Negative Valve Overlap (NVO) is a potential control strategy for enabling Low-Temperature Gasoline Combustion (LTGC) at low loads. While the thermal effects of NVO fueling on main combustion are well-understood, the chemical effects of NVO in-cylinder fuel reforming have not been extensively studied. The objective of this work is to examine the effects of fuel molecular structure on NVO fuel reforming using gas sampling and detailed speciation by gas chromatography. Engine gas samples were collected from a single-cylinder research engine at the end of the NVO period using a custom dump-valve apparatus. Six fuel components were studied at two injection timings: (1) iso-octane, (2) n-heptane, (3) ethanol, (4) 1-hexene, (5) cyclohexane, and (6) toluene. All fuel components were studied neat except for toluene - toluene was blended with 18.9% nheptane by liquid volume to increase the fuel reactivity.

Pulsed nanosecond discharges (PND) can achieve ignition in internal combustion engines through enhanced reaction kinetics as a result of elevated electron energies without the associated increases in translational gas temperature that cause electrode erosion. Atomic oxygen (O), including its electronically excited states, is thought to be a key species in promoting low-temperature ignition. In this paper, high-voltage (17-24 kV peak) PND are examined in oxygen/nitrogen/carbon dioxide/water mixtures at engine-relevant densities (up to 9.1 kg/m3) through pressure-rise calorimetry and direct imaging of excited-state O-atom and molecular nitrogen (N2) in an optically accessible spark calorimeter, with the anode/cathode gap distance set to 5 mm or with an anode-only configuration (DC corona). The conversion efficiency of pulse electrical energy into thermal energy was measured for PND with secondary streamer breakdown (SSB) and similar low-temperature plasmas (LTP) without.

Two-dimensional planar imaging and one-dimensional, spectrally-resolved line-imaging of laser-induced fluorescence from CO and UHC are performed to help identify the sources of these emissions in a light-duty diesel engine operating in a partially-premixed compression ignition combustion regime. Cycle-averaged measurements are made in the clearance volume above the piston crown at a 3 bar IMEP, 1500 rpm baseline operating condition. Sweeps of injection timing, load, and O2 concentration are performed to examine the impact of these parameters on the in-cylinder spatial distributions of CO and UHC. At the baseline operating condition, the main contributions to UHC from the clearance volume stem from regions near the cylinder centerline and near the cylinder wall, where UHC likely emanates from the top ring-land crevice. Broadly distributed CO within the squish volume dominates over CO observed near the cylinder centerline.

Pre-chamber ignition has demonstrated capability to increase internal combustion engine in-cylinder burn rates and enable the use of low engine-out pollutant emission combustion strategies. In the present study, newly designed passive pre-chambers with different nozzle-hole patterns - that featured combinations of radial and axial nozzles - were experimentally investigated in an optically accessible, single-cylinder research engine. The pre-chambers analyzed had a narrow throat geometry to increase the velocity of the ejected jets. In addition to a conventional inductive spark igniter, a nanosecond spark ignition system that promotes faster early burn rates was also investigated. Time-resolved visualization of ignition and combustion processes was accomplished through high-speed hydroxyl radical (OH*) chemiluminescence imaging. Pressure was measured during the engine cycle in both the main chamber and pre-chamber to monitor respective combustion progress.

The impact of 50 ppm intake seeding of ozone (O3) on performance and emissions characteristics was explored in a single-cylinder research engine operated under lean spark assisted compression ignition (SACI) conditions. Optical access into the engine enabled complementary crank angle resolved measurements of in-cylinder O3 concentration via ultraviolet (UV) light absorption. Experiments were performed at moderate loads (4 - 5 bar indicated mean effective pressure) and low-to-moderate engine speeds (800 - 1400 revolutions per minute). Each operating condition featured a single early main injection and maximum brake torque spark timing. Intake pressure was fixed at 1.0 bar, while intake temperatures were varied between 42 - 80 °C. Moderate amounts of internal residuals (12 - 20%) were retained through the use of positive valve overlap. Ozone addition was to found stabilize combustion relative to similar conditions without O3 addition by promoting end gas auto-ignition.

Performance and emissions characteristics were measured for a part- load operating point using an optically-accessible single-cylinder gasoline research engine equipped with three different exploratory nanosecond repetitively pulse discharge (NRPD) igniters. The three igniters investigated are as follows: 1) a four-prong advanced corona ignition system (ACIS) that produces large ignition volumes from streamer discharges, 2) a barrier discharge igniter (BDI) that generates strong surface plasma along the insulator that completely encases the power electrode, and 3) a J-hook non-resistive nanosecond spark (NRNS) igniter. For select conditions, high-speed imaging (20 kHz) of excited state hydroxyl (OH*) chemiluminescence was performed to measure flame development in-cylinder. An available NRPD pulse generator was used to supply positive direct current (DC) pulses (~ 10 ns pulse width) to each igniter at a fixed 100 kHz frequency.

The influence of early induction stroke direct injection on late-cycle flows was investigated for a lean-burn, high-tumble, gasoline engine. The engine features side-mounted injection and was operated at a moderate load (8.5 bar brake mean effective pressure) and engine speed (2000 revolutions per minute) condition representative of a significant portion of the duty cycle for a hybridized powertrain system. Thermodynamic engine tests were used to evaluate cam phasing, injection schedule, and ignition timing such that an optimal balance of acceptable fuel economy, combustion stability, and engine-out nitrogen oxide (NOx) emissions was achieved. A single cylinder of the 4-cylinder thermodynamic engine was outfitted with an endoscope that enabled direct imaging of the spark discharge and early flame development.