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Selective Catalytic Reduction (SCR) is the dominant solution for meeting future NOx reduction regulations for heavy-duty diesel powertrains. SCR systems benefit from closed-loop control if an appropriate exhaust gas sensor were available. An ammonia sensor has recently been developed for use as a feedback element in closed-loop control of urea dosing in a diesel SCR aftertreatment system. Closed-loop control of SCR dosing enables the SCR system to be robust against disturbances and to meet conformity of production (COP) and in-use compliance norms. The ammonia sensor is based on a non-equilibrium electrochemical principle and outputs emf signals. The sensor performs well when tested in a diesel engine exhaust environment and has minimum cross interference with CO, HC, NO, NO2, SO2, H2O and O2. Previous work, done in a simulation environment, demonstrated that an ammonia sensor provides the optimal feedback for urea dosing control algorithms in closed-loop SCR systems.