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Sources of unburned hydrocarbon (UHC) emissions are examined for a highly dilute (10% oxygen concentration), moderately boosted (1.5 bar), low load (3.0 bar IMEP) operating condition in a single-cylinder, light-duty, optically accessible diesel engine undergoing partially-premixed low-temperature combustion (LTC). The evolution of the in-cylinder spatial distribution of UHC is observed throughout the combustion event through measurement of liquid fuel distributions via elastic light scattering, vapor and liquid fuel distributions via laser-induced fluorescence, and velocity fields via particle image velocimetry (PIV). The measurements are complemented by and contrasted with the predictions of multi-dimensional simulations employing a realistic, though reduced, chemical mechanism to describe the combustion process.

Low temperature combustion (LTC) strategies, which can mitigate emissions of particulate matter (PM) and nitrogen oxides (NOx) from diesel engines, typically have longer ignition delays compared to conventional diesel operation. With extended ignition delays, more time is available for premixing, which reduces PM formation. The effect of varying ignition delay on the spatial and temporal evolution of soot in LTC diesel jets is studied by imaging the natural soot luminosity, while the in-cylinder soot mass and temperature are measured using two-color soot thermometry. Ignition delay in the engine is controlled by adjusting the intake air temperature while keeping the same charge density at TDC. This allowed us to study sooting characteristics at various ignition delays while keeping the same diesel jet penetration for all the cases.

The soot distribution as function of ambient O₂ mole fraction in a heavy-duty diesel engine was investigated at low load (6 bar IMEP) with laser-induced incandescence (LII) and natural luminosity. A Multi-YAG laser system was utilized to create time-resolved LII using 8 laser pulses with a spacing of one CAD with detection on an 8-chip framing camera. It is well known that the engine-out smoke level increases with decreasing oxygen fraction up to a certain level where it starts to decrease again. For the studied case the peak occurred at an O₂ fraction of 11.4%. When the oxygen fraction was decreased successively from 21% to 9%, the initial soot formation moved downstream in the jet. At the lower oxygen fractions, below 12%, no soot was formed until after the wall interaction. At oxygen fractions below 11% the first evidence of soot is in the recirculation zone between two adjacent jets.

This paper presents experimental results for two fuel-related topics in a diesel engine: (1) how fuel volatility affects the premixed burn and heat release rate, and (2) how ignition quality influences the soot formation. Fast evaporation of fuel may lead to more intense heat release if a higher percentage of the fuel is mixed with air to form a combustible mixture. However, if the evaporation of fuel is driven by mixing with high-temperature gases from the ambient, a high-volatility fuel will require less oxygen entrainment and mixing for complete vaporization and, consequently, may not have potential for significant heat release simply because it has vaporized. Fuel cetane number changes also cause uncertainty regarding soot formation because variable ignition delay will change levels of fuel-air mixing prior to combustion.

The effects of spray targeting on mixing, combustion, and pollutant formation under a low-load, late-injection, low-temperature combustion (LTC) diesel operating condition are investigated by optical engine measurements and multi-dimensional modeling. Three common spray-targeting strategies are examined: conventional piston-bowl-wall targeting (152° included angle); narrow-angle floor targeting (124° included angle); and wide-angle piston-bowl-lip targeting (160° included angle). Planar laser-induced fluorescence diagnostics in a heavy-duty direct-injection optical diesel engine provide two-dimensional images of fuel-vapor, low-temperature ignition (H2CO), high-temperature ignition (OH) and soot-formation species (PAH) to characterize the LTC combustion process.

Multiple fuel-injections during a single engine cycle can reduce combustion noise and improve pollutant emissions tradeoffs. Various hypotheses have been proposed in the literature regarding the in-cylinder processes responsible for the pollutant emissions improvements. This paper provides a brief overview of these hypotheses along with an investigation exploring which of these mechanisms are important for post injections under low-temperature combustion (LTC) conditions in a heavy-duty diesel engine. In-cylinder soot and exhaust smoke are measured by 2-color soot thermometry and filter paper blackening, respectively. The evolution and interaction of soot regions from each of the injections is visualized using high-speed imaging of soot luminosity, both in the piston bowl and in the squish regions.

The influence of soy- and palm-based biofuels on the in-cylinder sources of unburned hydrocarbons (UHC) and carbon monoxide (CO) was investigated in an optically accessible research engine operating in a partially premixed, low-temperature combustion regime. The biofuels were blended with an emissions certification grade diesel fuel and the soy-based biofuel was also tested neat. Cylinder pressure and emissions of UHC, CO, soot, and NOx were obtained to characterize global fuel effects on combustion and emissions. Planar laser-induced fluorescence was used to capture the spatial distribution of fuel and partial oxidation products within the clearance and bowl volumes of the combustion chamber. In addition, late-cycle (30° and 50° aTDC) semi-quantitative CO distributions were measured above the piston within the clearance volume using a deep-UV LIF technique.

The potential of boosted HCCI for achieving high loads has been investigated for intake pressures (Piⁿ) from 100 kPa (naturally aspirated) to 325 kPa absolute. Experiments were conducted in a single-cylinder HCCI research engine (0.98 liters) equipped with a compression-ratio 14 piston at 1200 rpm. The intake charge was fully premixed well upstream of the intake, and the fuel was a research-grade (R+M)/2 = 87-octane gasoline with a composition typical of commercial gasolines. Beginning with Piⁿ = 100 kPa, the intake pressure was systematically increased in steps of 20 - 40 kPa, and for each Piⁿ, the fueling was incrementally increased up to the knock/stability limit, beyond which slight changes in combustion conditions can lead to strong knocking or misfire. A combination of reduced intake temperature and cooled EGR was used to compensate for the pressure-induced enhancement of autoignition and to provide sufficient combustion-phasing retard to control knock.

Fuel injection during negative valve overlap offers a promising method of controlling HCCI combustion, but sorting out the thermal and chemical effects of NVO fueling requires knowledge of temperatures throughout the cycle. Computing bulk temperatures throughout closed portions of the cycle is relatively straightforward using an equation of state, once a temperature at one crank angle is established. Unfortunately, computing charge temperatures at intake valve closing for NVO operation is complicated by a large, unknown fraction of residual gases at unknown temperature. To address the problem, we model blowdown and recompression during exhaust valve opening and closing events, allowing us to estimate in-cylinder charge temperatures based on exhaust-port measurements. This algorithm permits subsequent calculation of crank-angle-resolved bulk temperatures and residual gas fraction over a wide range of NVO operation.

Measurements of ignition behavior, homogeneous reactor simulations employing detailed kinetics, and quantitative in-cylinder imaging of fuel-air distributions are used to delineate the impact of temperature, dilution, pilot injection mass, and injection pressure on the pilot ignition process. For dilute, low-temperature conditions characterized by a lengthy ignition delay, pilot ignition is impeded by the formation of excessively lean mixture. Under these conditions, smaller pilot mass or higher injection pressures further lengthen the pilot ignition delay. Similarly, excessively rich mixtures formed under relatively short ignition delay conditions typical of conventional diesel combustion will also prolong the ignition delay. In this latter case, smaller pilot mass or higher injection pressures will shorten the ignition delay. The minimum charge temperature required to effect a robust pilot ignition event is strongly dependent on charge O2 concentration.

Despite ongoing research efforts directed at reducing engine-out emissions, diesel engines are known to be one of the largest sources of atmospheric particulate matter (i.e., soot). Quantitative measurements are of primary importance to address soot production during the combustion process in the cylinder of diesel engines. This study presents the capabilities of an extinction-based diagnostic developed to quantitatively measure the soot volume fraction in n-dodecane sprays injected in a high-pressure, high-temperature vessel. Coupled with high-speed imaging, the technique yields time-resolved measurements of the soot field by relying on a diffused back-illumination scheme to improve extinction quantification in the midst of intense beam steering. The experiments performed in this work used two wavelengths, which, when combined with the Rayleigh-Debye-Gans theory, provide information about the optical and physical properties of soot.

Although soot-formation processes in diesel engines have been well characterized during the mixing-controlled burn, little is known about the distribution of soot throughout the combustion chamber after the end of appreciable heat release during the expansion and exhaust strokes. Hence, the laser-induced incandescence (LII) diagnostic was developed to visualize the distribution of soot within an optically accessible single-cylinder direct-injection diesel engine during this period. The developed LII diagnostic is semi-quantitative; i.e., if certain conditions (listed in the Appendix) are true, it accurately captures spatial and temporal trends in the in-cylinder soot field. The diagnostic features a vertically oriented and vertically propagating laser sheet that can be translated across the combustion chamber, where “vertical” refers to a direction parallel to the axis of the cylinder bore.

Well-mixed lean SI engine operation can provide improvements of the fuel economy relative to that of traditional well-mixed stoichiometric SI operation. This work examines the use of two methods for improving the stability of lean operation, namely multi-pulse transient plasma ignition and intake air preheating. These two methods are compared to standard SI operation using a conventional high-energy inductive ignition system without intake air preheating. E85 is the fuel chosen for this study. The multi-pulse transient plasma ignition system utilizes custom electronics to generate 10 kHz bursts of 10 ultra-short (12ns), high-amplitude pulses (200 A). These pulses were applied to a custom spark plug with a semi-open ignition cavity. High-speed imaging reveals that ignition in this cavity generates a turbulent jet-like early flame spread that speeds up the transition from ignition to the main combustion event.

Flow field asymmetry can lead to an asymmetric mixture preparation in Diesel engines. To understand the evolution of this asymmetry, it is necessary to characterize the in-cylinder flow over the full compression stroke. Moreover, since bowl-in-piston cylinder geometries can substantially impact the in-cylinder flow, characterization of these flows requires the use of geometrically correct pistons. In this work, the flow has been visualized via a transparent piston top with a realistic bowl geometry, which causes severe experimental difficulties due to the spatial and temporal variation of the optical distortion. An advanced optical distortion correction method is described to allow reliable particle image velocimetry (PIV) measurements through the full compression stroke. Based on the ensemble-averaged velocity results, flow asymmetry characterized by the swirl center offset and the associated tilting of the vortex axis is quantified.

The major challenge of the post-processing of soot aggregates in transmission electron microscope (TEM) images is the detection of soot primary particles that have no clear boundaries, vary in size within the fractal aggregates, and often overlap with each other. In this study, we propose an automated detection code for primary particles implementing the Canny Edge Detection (CED) and Circular Hough Transform (CHT) on pre-processed TEM images for particle edge enhancement using unsharp filtering as well as image inversion and self-subtraction. The particle detection code is tested for soot TEM images obtained at various ambient and injection conditions, and from five different combustion facilities including three constant-volume combustion chambers and two diesel engines.

Leaner lifted-flame combustion (LLFC) is a mixing-controlled combustion strategy for compression-ignition (CI) engines that does not produce soot because the equivalence ratio at the lift-off length is less than or equal to approximately two. In addition to completely preventing soot formation, LLFC can simultaneously control emissions of nitrogen oxides because it is tolerant to the use of exhaust-gas recirculation for lowering in-cylinder temperatures. Experiments were conducted in a heavy-duty CI engine that has been modified to provide optical access to the combustion chamber, to study whether LLFC is facilitated by an oxygenated fuel blend (T50) comprising a 1:1 mixture by volume of tri-propylene glycol mono-methyl ether with an ultra-low-sulfur #2 diesel emissions-certification fuel (CFA). Results from the T50 experiments are compared against baseline results using the CFA fuel without the oxygenate.

The 4th Workshop of the Engine Combustion Network (ECN) was held September 5-6, 2015 in Kyoto, Japan. This manuscript presents a summary of the progress in experiments and modeling among ECN contributors leading to a better understanding of soot formation under the ECN “Spray A” configuration and some parametric variants. Relevant published and unpublished work from prior ECN workshops is reviewed. Experiments measuring soot particle size and morphology, soot volume fraction (fv), and transient soot mass have been conducted at various international institutions providing target data for improvements to computational models. Multiple modeling contributions using both the Reynolds Averaged Navier-Stokes (RANS) Equations approach and the Large-Eddy Simulation (LES) approach have been submitted. Among these, various chemical mechanisms, soot models, and turbulence-chemistry interaction (TCI) methodologies have been considered.

The downsizing of internal combustion engines to increase fuel economy leads to challenges in both obtaining ignition and stabilizing combustion at boosted intake pressures and high exhaust gas recirculation dilution conditions. The use of non-thermal plasma ignition technologies has shown promise as a means to more reliably ignite dilute charge mixtures at high pressures. Despite progress in fundamental research on this topic, both the capabilities and operation implications of emerging non-thermal plasma ignition technologies in internal combustion engine applications are not yet fully explored. In this work, we document the effects of using a corona discharge ignition system in a single cylinder gasoline direct injection research engine relative to using a traditional inductive spark ignition system under conditions associated with both naturally aspirated (8 bar BMEP) and boosted (20 bar BMEP) loads at moderate (2000 rpm) and high (4000 rpm) engine speeds.

One way to develop an understanding of soot formation and oxidation processes that occur during direct injection and combustion in an internal combustion engine is to image the natural luminosity from soot over time. Imaging is possible when there is optical access to the combustion chamber. After the images are acquired, the next challenge is to properly interpret the luminous distributions that have been captured on the images. A major focus of this paper is to provide guidance on interpretation of experimental images of soot luminosity by explaining how radiation from soot is predicted to change as it is transmitted through the combustion chamber and to the imaging. The interpretations are only limited by the scope of the models that have been developed for this purpose. The end-goal of imaging radiation from soot is to estimate the amount of soot that is present.

Combustion issued from an eight-hole, direct-injection spray was experimentally studied in a constant-volume pre-burn combustion vessel using simultaneous high-speed diffused back-illumination extinction imaging (DBIEI) and OH* chemiluminescence. DBIEI has been employed to observe the liquid-phase of the spray and to quantitatively investigate the soot formation and oxidation taking place during combustion. The fuel-air mixture was ignited with a plasma induced by a single-shot Nd:YAG laser, permitting precise control of the ignition location in space and time. OH* chemiluminescence was used to track the high-temperature ignition and flame. The study showed that increasing the delay between the end of injection and ignition drastically reduces soot formation without necessarily compromising combustion efficiency. For long delays between the end of injection and ignition (1.9 ms) soot formation was eliminated in the main downstream charge of the fuel spray.