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A tracer laser-induced fluorescence (LIF) technique for the visualisation of fuel distribution in the presence of oxygen was developed and then used sequentially with high speed chemiluminescence imaging to study the correlation between the mixing and auto-ignition processes of high pressure Diesel jets. A single hole common rail Diesel injector allowing high injection pressures up to 150MPa was used. The reacting fuel spray was observed in a high pressure, high temperature cell that reproduces the thermodynamic conditions which exist in the combustion chamber of a Diesel engine during injection. Both free jet and flat wall impinging jet configurations were studied. Several tracers were first considered with the objective of developing a tracer-LIF technique in the presence of oxygen. 5-nonanone was selected for its higher fluorescence efficiency.

Penetration and combustion of fuel sprays is studied in conditions similar to gasoline direct injection engines. A closed pressurized and heated injection cell is used. It is equipped with quartz windows providing large optical accesses. A homogeneous flammable mixture is introduced in the cell and ignited to raise the internal pressure and temperature. Liquid fuel is injected at the time when the desired thermodynamic conditions are reached. Conditions representative of late injection in a direct-injection engine are selected. Gasoline spray ignition and combustion is provided by a spark plug with long electrodes, locating the electrode gap right in the middle of the spray. The combustion does not reach the wall, which makes this experiment interesting for the validation of combustion in CFD codes. Two pressure swirl injectors with spray angles of 60 and 90 degree are used. The fuel is iso-octane with 5% 3-pentanone as tracer.

The influence of piston geometry on the in-cylinder mixture distribution and combustion process in an optically-accessible, direct injection HCCI Diesel engine has been investigated. A new, purpose-designed piston which allows optical access directly into the combustion chamber bowl permitted the application of a number of optical diagnostic techniques. Firstly, laser-induced exciplex fluorescence (LIEF) has been applied in order to characterize the fuel spray and vapor development within the piston bowl. Subsequently a detailed study of the auto-ignition and two-stage Diesel HCCI combustion process has been conducted by a combination of direct chemiluminescence imaging, laser-induced fluorescence (LIF) of the intermediate species formaldehyde (CH2O) which is present during the cool flame and LIF of the OH radical later present in the reaction and burned gas zones at higher temperature.