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The simultaneous reduction of engine-out nitrogen oxide (NOx) and particulate emissions via low-temperature combustion (LTC) strategies for compression-ignition engines is generally achieved via the use of high levels of exhaust gas recirculation (EGR). High EGR rates not only result in a drastic reduction of combustion temperatures to mitigate thermal NOx formation but also increases the level of pre-mixing thereby limiting particulate (soot) formation. However, highly pre-mixed combustion strategies such as LTC are usually limited at higher loads by excessively high heat release rates leading to unacceptable levels of combustion noise and particulate emissions. Further increasing the level of charge dilution (via EGR) can help to reduce combustion noise but maximum EGR rates are ultimately restricted by turbocharger and EGR path technologies.

Single cylinder optical engines are used for internal combustion (IC) engine research as they allow for the application of qualitative and quantitative non-intrusive, diagnostic techniques to study in-cylinder flow, mixing, combustion and emissions phenomena. Such experimental data is not only important for the validation of computational models but can also provide a detailed insight into the physical processes occurring in-cylinder which is useful for the further development of new combustion strategies such as gasoline homogeneous charge compression ignition (HCCI) and Diesel low temperature combustion (LTC). In this context, it is therefore important to ensure that the performance of optical engines is comparable to standard all-metal engines. A comparison of optical and all-metal engine combustion and emissions performance was performed within the present study.

Low temperature combustion is a promising way to reach low NOx emissions in Diesel engines but one of its drawbacks, in comparison to conventional Diesel combustion is the drastic increase of Unburned Hydrocarbons (UHC). In this study, the sources of UHC of a low temperature combustion system were investigated in both a standard, all-metal single-cylinder Diesel engine and an equivalent optically-accessible engine. The investigations were conducted under low load operating conditions (2 and 4 bar IMEP). Two piston bowl geometries were tested: a wall-guided and a more conventional Diesel chamber geometry. Engine parameters such as the start of injection (SOI) timing, the level of charge dilution via exhaust gas re-circulation (EGR), intake temperature, injection pressure and engine coolant temperature were varied. Furthermore, the level of swirl and the diameter of the injector nozzle holes were also varied in order to determine and quantify the sources of UHC.

The formation mechanisms of unburned hydrocarbons (HC) in low NOx, homogeneous type Diesel combustion have been investigated in both standard and optical access single cylinder engines operating under low load (2 and 4 bar IMEP) conditions. In the standard (i.e. non-optical) engine, parameters such as injection timing, intake temperature and global equivalence ratio were varied in order to analyse the role of bulk quenching on HC emissions formation. Laser-induced fluorescence (LIF) imaging of in-cylinder unburned HC within the bulk gases was performed on the optical-access engine. Furthermore, studies were performed in order to ascertain whether the piston top-land crevice volume contributes significantly to engine-out HC emissions. Finally, the role of piston-top fuel films and their impact on HC emissions was studied. This was investigated on the all-metal engine using two fuels of different volatilities.

Tracer laser induced fluorescence (LIF) imaging of piston-top fuel films has been performed within the combustion chamber of an optically-accessible, single cylinder Diesel engine. The first objective of the study was to adapt the tracer LIF technique so as to perform in-cylinder imaging of the fuel films under reacting (i.e. combustion) conditions. The results obtained in a wall-guided, combustion chamber operating under highly dilute, Diesel low temperature combustion (LTC) conditions reveal the significant presence of late-cycle piston-top fuel films. Furthermore, it is believed that these fuel films contribute to engine-out hydrocarbon (HC) emissions via a mechanism of flash boiling. An attempt was also made to evaluate the role of fuel volatility on fuel film lifetimes. This was achieved by using a 50/50 fuel mixture of two single component fuels whose boiling points correspond to moderately high and low volatility components of standard Diesel fuel.

An experimental investigation into the structure and flame propagation characteristics of stratified and homogeneous combustion has been performed in an optically-accessible, direct-injection spark ignition (DISI) engine using OH planar laser-induced fluorescence (PLIF) imaging. Homogeneous and stratified operation was achieved by employing either early or late injection timing strategies during the intake or compression stroke respectively. Planar LIF OH images obtained revealed that for stratified operation, the 3D structure of the combustion zone is highly inhomogeneous and is predominantly due to high fuel concentration gradients which are formed as a result of local fuel mixture stratification. The images reveal a combustion structure which suggests that the flame propagation pathway is ultimately determined by the presence of these local fuel mixture inhomogeneities.

Planar laser-induced fluorescence (LIF) imaging of formaldehyde (CH2O) and OH has been performed to investigate the homogeneous charge, compression ignition (HCCI) combustion process inside the piston bowl of an optically-accessible, direct injection Diesel-fueled HCCI engine. In particular, the effects of charge dilution and the adoption of single and split injection strategies on the two-stage HCCI combustion have been studied. Results obtained show that the level of exhaust gas recirculation (EGR) significantly affects the pre-combustion or so called cool flame phase during which formaldehyde is detected. The cool flame phasing as indicated by the formation of this intermediate species is unaffected by the EGR level however, auto-ignition timing which marks the start of main combustion is inevitably advanced following a reduction in EGR and this ultimately determines the formaldehyde lifetime and consequently the degree of homogeneity attained.

The influence of piston geometry on the in-cylinder mixture distribution and combustion process in an optically-accessible, direct injection HCCI Diesel engine has been investigated. A new, purpose-designed piston which allows optical access directly into the combustion chamber bowl permitted the application of a number of optical diagnostic techniques. Firstly, laser-induced exciplex fluorescence (LIEF) has been applied in order to characterize the fuel spray and vapor development within the piston bowl. Subsequently a detailed study of the auto-ignition and two-stage Diesel HCCI combustion process has been conducted by a combination of direct chemiluminescence imaging, laser-induced fluorescence (LIF) of the intermediate species formaldehyde (CH2O) which is present during the cool flame and LIF of the OH radical later present in the reaction and burned gas zones at higher temperature.