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The main objective of this paper is to investigate the influence of injection pressures and fuel temperatures on the secondary injection spray evolution at the end of injection from a multi-hole gasoline direct injection (GDI) injector by Mie-scattering technique. The results of this paper show that the overall injection process can be classified into five stages which are injection delay stage, main injection stage, dwell stage, secondary injection stage and ligaments breakup stage respectively. Especially, the secondary injection occurs at the end of main injection, which is abnormal and undesirable spray behaviors. During the injection, big droplets and ligaments are injected through nozzle orifices at low speed. As the injection pressure increases, the phase of the secondary injection advances, and the injection duration decreases. At medium injection pressures (at 6, 8 MPa), more quantity of fuel are injected as ligaments.

The evolution of surface functional groups (SFGs) and the graphitization degree of soot generated in premixed methane flames are studied and the correlation between them is discussed. Test soot samples were obtained from an optimized thermophoretic sampling system and probe sampling system. The SFGs of soot were determined by Fourier transform infrared spectroscopy (FT-IR) and X-ray photoelectron spectroscopy (XPS) after removing the soluble impurities from the soot samples, while the graphitization degree of soot was characterized by Raman spectrum and electron energy loss spectroscopy (EELS). The results reveal that the number of aliphatic C-H groups and C=O groups shows an initial increase and then decrease in the sooting history. The large amount of aliphatic C-H groups and small amount of aromatic C-H groups in the early stage of the soot mass growth process indicate that aliphatic C-H groups make a major contribution to the early stage of soot mass growth.