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The conventional crash box with thin-walled column conceals some limitations on pedestrian protection and lightweight. The metallic NPR metamaterials designed in this study are based on re-entrant lattice structures. Re-entrant structures are known to be one main class of axenic structures that display negative Poisson’s ratio (NPR), which can be manufactured by 3D printing technology. This kind of metamaterial has good designability and can be used as the filling structure of the crash box to improve the crashworthiness of the car. This paper starts from the relations between geometric parameters of the metamaterial. Considering the deformation characteristics of the crash box, the structure were designed into some gradient types. The mechanical properties of different gradient structures under the same impact conditions were compared to find the proper gradient structures. Based on the studies, the gradient lattice structure is applied to the automobile crash box.