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In order to clarify future automobile technologies and fuel qualities to improve air quality, second phase of Japan Clean Air Program (JCAPII) had been conducted from 2002 to 2007. Predicting improvement in air quality that might be attained by introducing new emission control technologies and determining fuel qualities required for the technologies is one of the main issues of this program. Unregulated material WG of JCAPII had studied unregulated emissions from gasoline and diesel engines. Eight gaseous hydrocarbons (HC), four Aldehydes and three polycyclic aromatic hydrocarbons (PAHs) were evaluated as unregulated emissions. Specifically, emissions of the following components were measured: 1,3-Butadiene, Benzene, Toluene, Xylene, Ethylbenzene, 1,3,5-Trimethyl-benzene, n-Hexane, Styrene as gaseous HCs, Formaldehyde, Acetaldehyde, Acrolein, Benzaldehyde as Aldehydes, and Benzo(a)pyrene, Benzo(b)fluoranthene, Benzo(k)fluoranthene as PAHs.

The superior fuel economy of diesel engines compared to gasoline engines is favorable in reducing carbon dioxide (CO2) emissions. On the other hand, the reductions in nitrogen oxides (NOx) and particulate matter (PM) emissions are technically difficult, thus the improvement in the emission reduction technologies is important. Although the cooled exhaust gas recirculation (cooled-EGR) is the effective method to reduce NOx emissions, it is known to have durability and reliability problems, especially of the increased wear of piston rings and cylinder liners. Therefore, the degree of cooling and amount of EGR are both limited. To apply the cooled-EGR more effectively, the wear reduction technology for such components are indispensable. In this study, the negative effects of cooled-EGR on the wear are quantified by using a heavy-duty diesel engine, and its wear mechanism is identified.

Since in-cylinder flame temperature has a direct effect on an engine's NOx characteristics, these phenomena have been studied in detail in a DI diesel engine using a newly developed method allowing the in-cylinder temperature distribution to be measured by the two color method. The flame light introduced from the visualized combustion chamber of the engine is divided into two colors by filters. The images of combustion phenomena using the two wavelengths are recorded with a framing streak camera which includes a CCD camera. The flame temperature is immediately calculated by a computer using two color images from the CCD camera. A parameter study was then carried out to determine the influence of intake valve number of the engine, and fuel injection rate (pilot injection) on the in-cylinder temperature distribution.

To reduce ultra fine particle number concentration from a heavy-duty diesel engine, the effects of diesel fuel property and after-treatment systems were studied. The reduction of ultra fine particle number concentration over steady state mode using an 8 liter turbocharged and after-cooled diesel engine was evaluated. PM size distribution was measured by a scanning mobility particle sizer (SMPS). The evaluation used a commercially available current diesel fuel (Sulfur Content: 0.0036 wt%), high sulfur diesel fuel (Sulfur Content: 0.046 wt%) and low sulfur diesel fuel (Sulfur Content: 0.007 wt%). The after-treatment systems were an oxidation catalyst, a wire-mesh type DPF (Diesel Particle Filter) and a wall-flow type catalyzed DPF. The results show that fine particle number concentration is reduced with a low sulfur fuel, an oxidation catalyst, a wire-mesh type DPF (Diesel Particulate Filter) and wall flow type catalyzed DPF, respectively.

To reduce NOx and Particulate Matter (PM) emissions from a heavy-duty diesel engine, the effects of urea selective catalytic reduction (SCR) systems were studied. Proto type urea SCR system was composed of NO oxidation catalyst, SCR catalyst and ammonia (NH3) reduction catalyst. The NOx reduction performance of urea SCR system was improved by a new zeolite type catalyst and mixer for urea distribution at the steady state operating conditions. NOx and PM reduction performance of the urea SCR system with DPF was evaluated over JE05 mode of Japan. The NOx reduction efficiency of the urea SCR catalyst system was 72% at JE05 mode. The PM reduction efficiency of the urea SCR catalyst system with DPF was 93% at JE05 mode. Several kinds of un-regulated matters were detected including NH3 and N2O leak from the exhaust gas. It is necessary to have further study for detailed measurements for un-regulated emissions from urea solution.

To reduce NOx emissions from a heavy-duty engine at low exhaust temperature conditions, the plasma-assisted SCR (Selective Catalytic Reduction) system was evaluated. The plasma-assisted SCR system is mainly composed of an ammonia gas supply system and a plasma reactor including a pellet type SCR catalyst. The preliminary test with simulated gases of diesel exhaust showed an improvement in the NOx reduction performance by means of the plasma-assisted SCR system, even below 150°C conditions. Furthermore, NOx reduction ratio was improved up to 77% at 110°C with increase in the catalyst volume. Also NOx emissions from a heavy-duty diesel engine over the transient test mode in Japan (JE05) were reduced by the plasma-assisted SCR system. However, unregulated emissions, e.g., aldehydes, were increased with the plasma environment. This paper reports the advantages and disadvantages of the plasma-assisted SCR system for a heavy-duty diesel engine.

The Hino E13C was developed for heavy-duty truck application to meet Japan's 2003 NOx and 2005 particulate emissions standards simultaneously with significant fuel economy improvement. A combined EGR system consisting of an external EGR system with a highly efficient EGR cooler and an internal EGR system with an electronically controlled valve actuation device was newly developed to reduce NOx emissions for all operating conditions without requiring a larger engine coolant radiator. A Hino-developed DPR was installed to achieve extremely low particulate emissions at the tail pipe. Increased strength of engine structural components and a ductile cast iron piston enabled high BMEP operation at lower engine speeds and reductions of both engine size and weight. This paper describes key technologies developed for the E13C as well as the development results.

Diesel emissions are significant issue worldwide, and emissions requirements have become so tough that. the application of after-treatment systems is now indispensable in many countries To meet even more stringent future emissions requirements, it has become apparent that the improvement of market fuel quality is essential as well as the development in engine and exhaust after-treatment technology. Japan Clean Air Program II (JCAP II) is being conducted to assess the direction of future technologies through the evaluation of current automobile and fuel technologies and consequently to realize near zero emissions and carbon dioxide (CO2) emission reduction. In this program, effects of fuel properties on the performance of diesel engines and a vehicle equipped with two types of diesel NOx emission after-treatment devices, a Urea-SCR system and a NOx storage reduction (NSR) catalyst system, were examined.

A 2-LEG NOx Storage-Reduction (NSR) catalyst system is one of potential after-treatment technology to meet stringent NOx and PM emissions standards as Post New Long Term (Japanese 2009 regulation) and US'10. Concerning NOx reduction using NSR catalyst, a secondary fuel injection is necessary to make fuel-rich exhaust condition during the NOx reduction, and causes its fuel penalty. Since fuel injected in the high-temperature (∼250 degrees Celsius) exhaust instantly reacts with oxygen in common diesel exhaust, the proportion of fuel consumption to reduce the NOx stored on NSR catalyst is relatively small. A 2-LEG NSR catalyst system has the decreasing exhaust flow mechanism during NOx reduction, and the potential to improve the NOx reduction and fuel penalty. Therefore, this paper studies the 2-LEG NSR catalyst system. The after-treatment system consists of NSR catalysts, a secondary fuel injection system, flow controlled valves and a Catalyzed Diesel Particulate Filter (CDPF).

This paper is an attempt to estimate the traffic demand of private vehicles in the Philippines and Thailand toward 2030. Estimation of road traffic volume is one of the most important elements for determining fuel consumption and emission gas levels. The level of passenger car ownership is still low, but there has been a distinct shift toward passenger cars due to the lack of mass transport. In Asian countries, inspection and maintenance and emission standards are the most important policy measures. The projections of car stock are evaluated as the emissions of PM, CO and NOx by applying these policy measures in the case of Thailand.

In the urea SCR system, urea solution is injected by injector installed in the front stage of the SCR catalyst, and NOx can be purified on the SCR catalyst by using NH3 generated by the chemical reaction of urea. NH3 is produced by thermolysis of urea and hydrolysis of isocyanic acid after evaporation of water in the urea solution. But, biuret and cyanuric acid which may cause deposit are sometimes generated by the chemical reactions without generating NH3. Spray behavior and chemical reaction of urea solution injected into the tail-pipe are complicated. The purpose of this study is to reveal the spray behavior and NH3 generation process in the tail-pipe, and to construct the model capable of predicting those accurately. In this report, the impingement spray behavior is clarified by scattered light method in high temperature flow field. Liquid film adhering to the wall and deposit generated after evaporation of water from the liquid film are photographed by the digital camera.

This work investigated the mechanism of oil dilution by post injection to remove accumulated particulate matter on the diesel particulate filter of diesel engines. We developed a model to simulate post injection spray under low ambient gas pressure conditions. The model can predict the quantity of fuel mass adhered on the cylinder wall. The adhered fuel enters oil sump through the piston ring and cause oil dilution. The fuel in diluted oil evaporates during normal engine operations. We focus on the mechanism of fuel evaporation from diluted oil. The effects of engine speed and oil temperature on the evaporation were investigated. The results showed that the fuel evaporation rate increases with increasing engine speed and oil temperature. Furthermore, we developed an empirical model to predict the fuel evaporation rate of diluted oil through regression analysis with measured data.

For the better understanding of nanoparticles observed on the rode side, adding to the emission test on the chassis dynamometer and engine dynamometer test, possible factors for formation of nanoparticles are investigated. As other possible factors, cold starting of transient test cycle, blow-by gas from heavy duty diesel engine without a positive crankcase ventilation, exhaust braking, and plume mixing of vehicle exhausts were investigated. Nuclei mode particles under the transient test cycles formed during fuel cut period, fuel enrichment period and idling period. Concentration of nuclei mode particles during the idling period are depends on exhaust temperature. The higher exhaust temperature courses the lower number concentration but variation range is within twice. Emission rate of nanoparticles from blow-by gas is one thousandth of tail pipe emissions rate and was found to be negligible.

Single cylinder engine testing was carried out to clearly understand the test results of multi-cylinder engines reported by the Diesel WG in JCAP (Japan Clean Air Program) (1), (2), (3) and (4). In this tests, engine specifications such as fuel injection pressure, nozzle hole diameter, turbo-charging pressure, EGR rate, and fuel properties such as 1-, 2-, 3-ring aromatics content, n-,i-paraffins content, and T90 were parametrically changed and their influence on the emissions were studied. PM emission generally increased in each engine condition with increased aromatic contents and T90. In particular, multi ring aromatics brought about large increases in PM regardless of the engine conditions. The influence of fuel properties on NOx emission is smaller than the influence on PM emission. Some other fuels that have various side chain structures of 1-ring aromatics, normal paraffins only and various naphthene contents were also investigated.

Newly designed laboratory measurement system, which reproduces particle number size distributions of both nuclei and accumulation mode particles in exhaust emissions, was developed. It enables continuous measurement of nano particle emissions in the size range between 5 and 1000 nm. Evaluations of particle number size distributions were conducted for diesel vehicles with a variety of emission aftertreatment devices and for gasoline vehicles with different combustion systems. For diesel vehicles, Diesel Oxidation Catalyst (DOC), urea-Selective Catalytic Reduction (urea-SCR) system and catalyzed Diesel Particulate Filter (DPF) were evaluated. For gasoline vehicles, Lean-burn Direct Injection Spark Ignition (DISI), Stoichiometric DISI and Multi Point Injection (MPI) were evaluated. Japanese latest transient test cycles were used for the evaluation: JE05 mode driving cycle for heavy duty vehicles and JC08 mode driving cycle for light duty vehicles.

Development is proceeding on catalysts which separate the NOx in lean exhaust gas by adsorption and then reduce the adsorbed NOx in combustion exhaust gas with the stoichiometric or a slightly richer air fuel ratio, as well as exhaust conversion technology that uses these catalysts. Amidst this research it has been found that catalysts containing mixed metal oxides exhibit superior NOx adsorption performance, so the authors prepared a mixed metal oxide catalyst by adding precious metals and promoters, etc. The resulting catalyst has high heat resistance and also offers excellent SOx durability. These properties were presumed to be due to an adsorbent including the mixed metal oxide, and the relation between the physical properties and NOx conversion properties of the catalyst was investigated.

Air Quality Modeling Working Group developed two models to evaluate effects of automobile emission reduction measures on air quality improvement: Urban Air Quality Simulation Model in which secondary aerosol formation processes have been incorporated, and Roadside Air Quality Simulation Model in which micro-scale traffic flow has been taken into consideration. Concretely, a model has been built up for estimating SPM concentration in ambient air in which high concentrated air pollutants have been contained during summer and winter. The model has been built up by using UAM (Urban Airshed Model) as base model, and the following modification has been made to the base model. First, ISSOROPIA (secondary inorganic aerosol equilibrium model) has been added to the base model, and a secondary organic aerosol formation/reaction model (SOA model) has been incorporated into the model.

This paper proposes a new mixing-controlled, low temperature combustion (LTC) approach for high-speed direct injection (HSDI) diesel engines. The purpose of this approach is to avoid the excessively high pressure-rise rate (PRR) of premixed, kinetics-controlled LTC and to enable the low nitrogen oxides (NOx) combustion to operate over the wide speed and load range of the engine. To address the soot/noise trade-off at high load LTC operating conditions, the pressure modulated multiple-injection coupled with swirl control was applied. This injection strategy enables the injection of high pressure (HP) main spray into the local high temperature region of the already burning low pressure (LP) pilot spray injected from the neighboring injection hole. By employing this injection strategy, the equivalence ratio (φ) distribution of mixture is drastically varied during main combustion processes.

We developed a thermal calculation 1D simulator for an electric valve timing control system (VTC). A VTC can optimize the open and close timing of the intake and exhaust valves depending on the driving situation. Since a conventional VTC is driven hydraulically, the challenges are response speed and operation limit at low temperature. Our company has been developing an electric VTC for quick response and expansion of operating conditions. Currently, it is necessary to optimize the motor and reduction gear design to balance quicker response with downsizing. Therefore, a coupled simulator that can calculate electricity, mechanics, control, and thermo characteristics is required. In 1D simulation, a thermal network method is commonly used for thermal calculation. However, an electric VTC is attached to the end of a camshaft; therefore, determining thermal resistances is difficult. We propose a method of determining thermal resistances, using both theoretical and experimental approaches.

A new combustion system targeting a drastic decrease in NOx emission and a brake specific energy consumption equivalent to that of a DI diesel engine has been developed. In this new combustion system, a lean burn system using early injection was employed to reduce NOx emission and an auto-ignition DI engine system was employed to achieve the low energy consumption. Methanol was used as the fuel for reducing NOx emission. The objective of this study is to clarify the possibility of the system for the auto-ignition of a premixed lean mixture of methanol fuel. This study shows that the gas temperature at ignition, Tig, is the predominant factor affecting auto-ignition. Auto-ignition occurs when Tig exceeds approximately 1000K. The methanol lean burn system in an auto-ignition DI engine drastically decreased NOx emission with almost the same brake specific energy consumption as a diesel engine in the middle load region.