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JSC-1A lunar simulant has been applied to AZ93 and AgFEP thermal control surfaces on aluminum substrates in a simulated lunar environment. The temperature of these surfaces was monitored as they were heated with a solar simulator using varying angles of incidence and cooled in a 30 K coldbox. Thermal modeling was used to determine the solar absorptivity (a) and infrared emissivity (e) of the thermal control surfaces in both their clean and dusted states. It was found that even a sub-monolayer of dust can significantly raise the α of either type of surface. A full monolayer can increase the α/ε ratio by a factor of 3–4 over a clean surface. Little angular dependence of the α of pristine thermal control surfaces for both AZ93 and AgFEP was observed, at least until 30° from the surface. The dusted surfaces showed the most angular dependence of α when the incidence angle was in the range of 25° to 35°.