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Reversible adsorption on zeolite molecular sieve material allows selective removal of carbon dioxide (CO2) from spacecraft air without the use of expendables. The four-bed molecular sieve (4BMS) CO2 removal subsystem chosen for use on space station is based on proven Skylab technology and provides continuous CO2 removal from the cabin atmosphere and concentration for further processing downstream or venting overboard. A 4BMS subsystem has also been chosen to remove CO2 from air in the Systems Integration Research Facility (SIRF) at NASA/Johnson Space Center (JSC). After installation in the SIRF in 1992, the subsystem underwent extensive testing in which cycle time, process air flow rate, and process air inlet CO2 composition were varied. In order to obtain performance data required for integration, the subsystem was operated under both nominal and off-nominal conditions. Results of this testing are presented.

The Shuttle Orbiter humidity control and carbon dioxide removal system for extended duration missions presently uses a solid amine called HS-C. This August, on board STS-62, a new solid amine called HS-C+ will be used. HS-C+ uses the same amine and the substrate material, but a different preparation process. Forty-seven breakthrough tests have been conducted to characterize the performance of HS-C+. CO2 partial pressure, bed temperature, and H2O partial pressure were varied. Eleven HS-C breakthrough tests were also run to provide a direct comparison. Under all conditions tested, HS-C+ outperformed HS-C. Both materials adsorb all CO2 and H2O available at the start of a test when the beds are fully desorbed. As the bed becomes partially loaded, the CO2 and H2O adsorption rates decrease rapidly. HS-C+ continues adsorbing all CO2 and H2O available for a longer time. Greater surface area on HS-C+ may cause the improved performance.