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This study investigates the effects of octane quality on the performance, i.e., acceleration and power, and fuel economy (FE) of one late model US vehicle, which is powered by a small displacement, turbocharged, gasoline direct injection (GDI) engine. The relative importance of the gasoline parameters Research and Motor Octane Number (RON and MON) in meeting the octane requirement of this engine to run at an optimum spark timing for the given demand was considered by evaluating the octane index (OI), where OI = (1-K) RON + K MON and K is a constant depending on engine design and operating conditions. Over wide open throttle (WOT) accelerations, the average K of this Pontiac Solstice was determined as −0.75, whereby a lower MON would give a higher OI, a higher knock resistance and better performance.