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Ammonia is one of the most useful compounds that react with NOx selectively on a catalyst, such as V2O5-TiO2, under oxygen containing exhaust gas. However ammonia cannot be stored because of its toxicity for the small power generator in populated areas or for the diesel vehicles. A new concept for NOx reduction in diesel engine using ammonia is introduced. This system is constructed from the hydrogen generator by fuel reformer, the ammonia synthesizer, SCR catalyst for NOx reduction and the gas injection system of reformed gas into the cylinder. Experimental results show that, the SCR catalyst provides a very high rate of NOx reduction, reformed gas injection into cylinder is very effective for particulate reduction. WHEN CONSIDERING INTERNAL COMBUSTION ENGINES of the 1990's the question of how to harmonize the engine with the natural environments is one of the greatest problems. The internal combustion engine changes a substance into energy via its explosive combustion.

The time of, and location where ignition first occurs in a diesel fuel spray were investigated in a rapid compression machine (RCM) using the two–dimensional techniques of silicone oil particle scattering imaging (SSI), and the planar laser induced fluorescence (LIF) of formaldehyde. Formaldehyde has been hypothesized to be one of the stable intermediate species marking the start of oxidation reactions in a transient spray under compression ignition conditions. In this study, the LIF images of the formaldehyde formed in a diesel fuel spray during ignition process have been successfully obtained for the first time by exciting formaldehyde with the 3rd harmonic of the Nd:YAG laser. SSI images of the vaporizing spray, and the LIF images of formaldehyde were obtained together with the corresponding time record of combustion chamber pressures at initial ambient temperatures ranging from 580 K to 790 K.

It is well known that increasing the fuel injection pressure is effective for improving the diesel engine combustion. While studying the characteristics of the high pressure fuel spray which is injected in a high pressure vessel, the authors found weak shock waves generating around the fuel spray. To investigate the shock waves effect on the fuel spray the authors measured the propagation speed and pressure amplitude as functions of the injection pressure and ambient pressure. The results indicate that shock waves are generated when the fuel injection speed exceeds the ambient sonic speed. Also it was found that the pressure amplitude of shock wave is approximately 10 % of the ambient pressure and the shock waves spread at a sonic speed. The above results make us think that, isn't it possible to use shock waves for combustion improvement.

The rate of air entrainment into the flame and the rate of heat release are thermodynamically calculated in a DI diesel engine: A two-zone model is proposed which uses as input data three measured values of cylinder pressure, flame temperature, and injection rate. The correlations between both rates under various conditions make it clear that the combustion during early and main periods of diffusion combustion is mainly controlled by air entrainment into the flame. The effects of injection pressure, piston configuration, and swirl intensity on the air entrainment are also studied. And the extent of mixing in the flame is evaluated by the equivalence ratio in the flame which is also obtained by the same model. The trends of exhausted NO and soot concentrations well correlate with the equivalence ratios in the flame and measured flame temperatures under all conditions studied.

Previous research in our laboratory has shown that NOx emissions can be sharply reduced by PREDIC (PRE-mixed lean DIesel Combustion), in which fuel is injected very early in the compression process. However some problems still remain, such as higher fuel consumption, a lack of ignition timing control, and a large increase in THC and CO, compared to conventional diesel combustion. Appropriate mixture formation is necessary to solve these problems. In this paper, the influence of mixture formation on PREDIC was investigated. It was found that the pintle type injection nozzle was shown to be suitable for PREDIC, because it produced a comparatively uniform mixture in the combustion chamber and avoided collision of the fuel spray with the cylinder liner. Modeling by the KIVA-II software package was carried out to improve our understanding of the mixture formation process.

This paper reports on research works of ACE towards the most appropriate injection and combustion system for heavy-duty direct injection diesel engines. Selected items for the study are the effect of nozzle hole diameter, injection rate pattern, swirl ratio, and supercharging under high pressure fuel injection. According to those experimental results, the combination of over 150MPa injection pressure with controlled injection rate, smaller nozzle hole diameter, and quiescent combustion systems shows the best performance and emission. The mechanisms of the combustion improvement are discussed from the turbulent mixing viewpoint, including the results of combustion observation.

Control of turbulence during the compression stroke is suggested by both theoretical calculations and experimental results obtained with an LDV measurement in a motored engine. The authors have found experimentally that when an axial distribution of swirl intensity exists, a large-scale annular vortex is formed inside the cylinder during the compression stroke and this vortex generates and transports turbulence energy. A numerical calculation is adopted to elucidate this phenomenon. Then, an axial stratification of swirl intensity is found to generate a large-scale annular vortex during the compression stroke by an interaction between the piston motion and the axial pressure gradient. The initial swirl profile is parametrically varied to assess its effect on the turbulence parameters. Among calculated results, turbulence energy is enhanced strongest when the swirl intensity is highest at the piston top surface and lowest at the bottom surface of the cylinder head.

A new model to describe diesel combustion process has been developed. In this model diesel combustion field is divided into two zones, premixing and combustion. Turbulent mixing process is described by the stochastic approach in each zone separately. Comparison of calculations with experimental results showed that this model can predict the entire course of heat release and nitrogen-oxide formation precisely, under wide-spread conditions. Two-dimensional flame temperature distributions in the combustion field by the two color method were compared with simulation results. Both the measured and the calculated flame temperature distributions showed good agreements with each other. In the diesel combustion process, the injected fuel mixes with air entrained inside the spray. The mixture is thus formed, and ignites at several points. Random expansion of flamelets accelerates both mixing and combustion. Following this, fairly moderate diffusion combustion proceeds.

The OH and soot in an unsteady flame, which was achieved in a rapid compression machine, were visualized simultaneously by the laser-induced fluorescence and laser-induced scattering techniques. The fuel mixture consisting of 90% paraffin hydrocarbon (reference fuel) and 10% polypropylene-glycol was used to reduce the optical attenuation caused by dense soot cloud. The simultaneous images of the fluorescence from OH and scattering from soot show that the soot and OH exist separately from each other in the leading portion of the spray flame, and the OH is formed earlier than the soot in the near field region of spray flame.

The rate of heat release of a free diesel flame was measured with a rapid compression machine which has a compression ratio of 14.7 and a combustion chamber with a diameter of 196 mm and a thickness of 40 mm. Basing on the experimental observations of the high speed photographs of the spray and flame, the authors proposed a phenomenological model for predicting the rate of heat release of the flame. The model consists of three basic models; air entrainment, mixing and combustion model. It was confirmed that the model could successively simulate the rate of heat release of a diesel flame in the quiescent chamber of the rapid compression machine.

The cross-sectional distribution of fuel vapor concentration in an evaporating spray was measured quantitatively by a new scattering imaging technique, silicone particle scattering imaging method, which was proposed in a previous paper[1]. When fuel containing silicone oil injected into a nitrogen environment at high temperature, the volatile base fuel in the droplets vaporized rapidly, leaving behind small droplets of silicone oil suspended in the vapor-gas mixture. The silicone oil droplets were illuminated by a thin laser sheet, and the scattered light was imaged by a CCD camera. The cross-sectional distribution of vapor concentration was estimated from the scattering image of the silicone oil droplets by Mie scattering theory. The results demonstrated clearly the inhomogeneity of the fuel vapor concentration. The distribution of vapor concentration was discontinuous, and islands of rich mixture with a scale of several millimeters existed in the center region of the spray.

A new method to determine simultaneously the temperature and the fuel vapor concentration inside an evaporating spray was described by using a laser-induced fluorescence technique. A TMPD doped base fuel composed of C12H26: 22%, C13H28: 54% and C14H30: 30% was injected into the combustion chamber of a rapid compression machine which is filled with a high temperature and high pressure nitrogen. The laser sheet was used for incident light, which was reflected by a prism located inside the combustion chamber and propagated through the center of an evaporating spray. The laser induced fluorescence intensity was imaged by a high speed-gated intensifier from a direction perpendicular to the incident light. The results shows that mixtures with high equivalence ratio are observed in the central region, while low equivalence ratio mixtures are observed in the periphery of the spray. It is also observed that the temperature of richest mixture is 50 K as low as the surrounding gas temperature.

A phenomenological model for predicting the rate of heat release of an axisymmetrical diesel flame which was achieved in a rapid compression machine has been proposed: Basing on the experimental observations, authors have introduced a new expression about the effects of abrupt thermal expansion due to the initial combustion on the air entrainment. A simple probability density function was also employed to express the distribution of the local equivalence ratio in the flame. The predicted rate of heat release showed good agreement with the experimental results in the diffusion combustion phase.

A theoretical model for predicting the evaporation process of liquid fuel sprays in both diesel and S.I. stratified charge engines is presented: The injected liquid fuel is assumed to break up into droplets with a certain time delay which is determined through careful experiments on the heat absorption process of injected fuel in a high temperature, high pressure inert atmosphere. The evaporation, heat absorption, and motion of these droplets are computed, together with the change of gas conditions inside the spray, by solving a coupled system of equations made up of heat and mass balance between droplets and gas. The effects of such parameters as the surrounding gas conditions, fuel properties, and spray characteristics on evaporation are investigated by the model. Reference is also made to the application of a predicted result to the calculation of burning rate in a direct injection diesel engine.

Some conceptual image of a diesel spray flame and its combustion promotion is shown based on the various interpretations of the enormous data obtained in our laboratory in these several years, on the flame temperature measurement by the two color method, the composition analysis by gas sampling, as well as the focus shadow photography, back illuminated photography and luminous photography by a high speed camera, on the diesel spray flame created in a large scale Rapid Compression Machine (diameter ϕ 200 mm thickness 40 mm) and a D-I engine (diameter (ϕ 95 mm)

Air-entrainment characteristics of non-evaporating sprays and flames were measured by means of high-speed photography including ordinary shadowgraphy of sprays, back diffused light illumination photography and laser shadow photography of flames. Effects of injection pressure and nozzle orifice diameter on air-entrainment characteristics were investigated parametrically. The amount of air entrained into a flame was calculated by a two-zone thermodynamic model with data obtained from the photographs and the pressure measurement in the combustion chamber. The air-entrainment characteristics of flames were compared with those of the corresponding sprays. It showed that immediately after the start of ignition, the air entrainment into a flame increased more rapidly as compared with the corresponding spray and then, with the development of diffusion combustion, the air entrainment gradually approached that of the spray.

To clarify the detailed structure of high pressure fuel spray, 2-D sectional images of non-evaporating fuel sprays in a high pressure vessel were observed by using the laser light sheet of a copper vapor laser. By this system, many sectional and continuous photographs of the same spray were obtained, and were very effective for the detailed observation of the spray inner structure and its developing process. The spray inner structure was very complicated, and its fuel density distribution was very heterogeneous. And for its developing process, the spray advances straight immediately after injected, then meanders, and deforms into a branch-like structure. Advancing downstream, these branches distribute complicatedly and heterogeneously with low density droplets. The heterogeneity is owing to these branches. And, the developing process is divided into four regions. Further, the effects of some parameters on this process were investigated.

To understand further the mixing process between the injected fuel and air in the combustion chamber of a diesel engine, the turbulent mixing process in a one-phase, two-dimensional transient jet was theoretically studied using the discrete vortex simulation. First, the simulation model was evaluated by comparisons between calculated and experimental data on two-dimensional turbulent jets. Second, the trajectories of the injected fluid elements marked with different colors were graphically demonstrated. Also the process of entrainment of the surrounding fluid into the jet was visually presented using colored tracers.

Several methods to reduce ignition delay period were tested in combination with a high pressure injection and effects on combustion improvement were examined. It was found that the reduction of ignition delay does not give so much improvement at the usual injection timing before TDC, but when the injection timing is considerably retarded or when the original ignition delay is relatively long, shortening of the ignition delay is effective to reduce pre-mixed combustion and NOx emission. Further, assuming the combustion system which conforms to the 1983 Japanese regulation as the reference system, it was found that the combination of pilot injection and high injection pressure, simultaneously reduces NOx by approximately 35% and smoke by 60-80% without worsening the fuel economy.

Soot concentration is very high in the periphery near the head of an unsteady spray flame which is achieved in a quiescent atmosphere in a rapid compression machine. To reduce soot concentration in this region, it was intended to improve fuel-air mixing by letting the flame impinge on a turbulence-generating plate. Two types of turbulence-generating plates, one donut-type, the other cross-type, were tested. Soot concentration in the flame was imaged using the laser shadow technique. The effect of injection pressure on soot reduction by the flame impingement was also investigated. The overall soot concentration is reduced significantly in the case when the flame impinges on the cross-type turbulence-generating plate at 50 mm (333 nozzle diameters) from the nozzle exit. The flame impingement on the cross-type turbulence-generating plate at 333 nozzle diameters makes soot reduction little dependent on injection pressures.