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A process to recover carbon fibers from obsolete polymer matrix composite (PMC) materials has been developed. Carbon fibers have been recovered from samples containing urethane-based or epoxy-based substrates. An experimental parametric study conducted on both the bench-scale and the pilot-scale has been done to determine the least-cost process conditions. Based on this study, we have evaluated process economics that suggested a payback of about one year. This process is also applicable to polymer matrix composite materials made with thermoplastic substrates. This paper presents the results of the experimental testing campaign and the results of the process economic analysis.

A sustainable activity is one that is economically attractive, environmentally friendly and provides a beneficial service to society in a safe and responsible manner. Having a sustainable operation is a target that today’s industries are striving to attain. The automotive industry and its products are major users of natural resources and a source of greenhouse emissions. In order to reduce its energy consumption and greenhouse emissions the industry is using more lightweighting materials in manufacturing its products. These materials include polymers, composites, aluminum and magnesium. The increased interest in hybrid vehicles will increase the need for new materials such as lithium, cobalt and nickel. At the same time, regulations are calling for recycling more of the obsolete vehicles. Replacing the steel, which is recyclable, with lighter materials will result in a reduction in the recycling rate of vehicles unless the lightweighting materials are recycled.

The process of shredding end-of-life vehicles to recover metals results in a byproduct commonly referred to as shredder residue. The four and a half million metric tons of shredder residue produced annually in the United States is presently land filled. To meet the challenges of automotive materials recycling, the U.S. Department of Energy is supporting research at Argonne National Laboratory in cooperation with the Vehicle Recycling Partnership (VRP) of the United States Council for Automotive Research (USCAR) and the American Plastics Council. This paper presents the results of a study that was conducted by Argonne to determine variations in the composition of shredder residue from different shredders. Over 90 metric tons of shredder residues were processed through the Argonne pilot plant. The contents of the various separated streams were quantitatively analyzed to determine their composition and to identify materials that should be targeted for recovery.

Over 250 million vehicles are operating on United States roads and highways and over 12 million of them reach the end of their useful lives annually. These end-of-life vehicles (ELVs) contain over 24 million tons (21.8 million metric tonnes) of materials including ferrous and non-ferrous metals, polymers, glass, and automotive fluids. They also contain many parts and components that are still useable and some that could be economically rebuilt or remanufactured. Dismantlers acquire the ELVs and recover from them parts for resale “as-is” or after remanufacturing. The dismantler then sells what remains of the vehicle, the “hulk”, to a shredder who shreds it to recover and sell the metals. Presently, the remaining non-metallic materials, commonly known as shredder residue, are mostly landfilled. The vehicle manufacturers, now more than ever, are working hard to build more energy efficient and safer, more affordable vehicles.