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Two-mode hybrid architectures with three planetary gear sets and four clutches will bring both flexibility and complexity to energy management of powertrains. In order to take full advantage of the increased degrees of freedom, highly delicate operation strategies are needed. We develop transmission efficiency models for power-split modes, and present a mode shift strategy assuming no battery power. When battery load leveling is additionally considered, the respective optimal operation set for each mode can be obtained and compared to yield a mode shift algorithm for general hybrid operation situations. The investigation of the strategies shows how frequently each mode is used, and verifies the effectiveness of fixed gear operations. We check the validity of the strategies by applying the algorithm to dynamic optimization and by predicting how it works during an actual driving simulation.