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Real world emissions are increasingly the standard of comparison for motor vehicle exhaust impact on the environment. The ability to collect such data has thus far relied primarily on full portable emissions measurement systems (PEMS) that are bulky, expensive, and time consuming to set up. The present work examines four compact, low cost, miniature PEMS (mPEMS) that offer the potential to expand our ability to record real world exhaust emissions over a larger number of operating conditions and combustion engine applications than currently possible within laboratory testing. It specifically addresses the particulate matter (PM) capabilities of these mPEMS, which employ three different methodologies for particle measurement: diffusion charger, optical scattering, and a multi-sensor approach that combines scattering, opacity, and ionization. Their performance is evaluated against solid particle number and PM mass with both vehicle tests and flame generated soot.

Pending reductions in light duty vehicle PM emissions standards from 10 to 3 mg/mi and below will push the limits of the gravimetric measurement method. At these levels the PM mass collected approaches the mass of non-particle gaseous species that adsorb onto the filter from exhaust and ambient air. This introduces an intrinsic lower limit to filter based measurement that is independent of improvements achieved in weighing metrology. The statistical variability of back-up filter measurements at these levels makes them an ineffective means for correcting the adsorption artifact. The proposed subtraction of a facility based estimate of the artifact will partially alleviate the mass bias from adsorption, but its impact on weighing variability remains a problem that can reach a significant fraction of the upcoming 3 and future 1 mg/mi standards. This paper proposes an improved PM mass method that combines the gravimetric filter approach with real time aerosol measurement.

This paper examines the issues concerning particulate matter (PM) emissions measurement at the 3 mg/mi level proposed as the future LEV III standard. These issues are general in nature, but are exacerbated at the low levels contemplated for upcoming emissions standards. They are discussed in the context of gasoline direct injection (GDI) engines, where they can have an important impact on the continued development of this technology for improved fuel economy. GDI particulate emissions, just as engine-out diesel PM, contain a high fraction of soot. But the total PM mass is significantly lower than from diesel engines, and there can be significant variations in emissions rate and apparent PM composition between cold-start and running emissions. PM emissions levels depend on sampling method and location. As a result, there can be substantial differences in PM sampled and diluted directly at the exhaust pipe, as opposed to measurements from a dilution tunnel.