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The effects of fuel octane have been assessed on the efficiency and emissions of a high compression ratio (ε=13) spark ignition direct injection (SIDI) engine. Under low load stratified operation (1200 rpm, ∼20% load), a low octane fuel (RON=84, comprised of toluene, iso-octane, and n-heptane) yielded higher brake thermal efficiency and significantly lower hydrocarbon emissions than a base gasoline (RON=91). The indicator diagram for the low octane fuel showed evidence for two stage heat release, suggesting the presence of spark induced compression ignition (SICI). These results suggest that higher efficiency under low load stratified conditions can be obtained with lower octane fuels that undergo SICI combustion. The effect of fuel octane under high load was assessed at WOT with a high RON model fuel (RON=103, comprised of toluene, iso-octane, and n-heptane).

Suppression or reduction of soot emissions is an important goal in the development of automotive engines for environmental and human health purposes. A better understanding at the molecular level of the formation process of soot particles resulting from collision and aggregation of smaller particles made of Polycyclic Aromatic Hydrocarbon (PAH) is needed. In addition to experiments, computational methods are efficient and valuable tools for this purpose. As a first step in our detailed computational chemistry study, we applied Ultra-Accelerated Molecular Dynamics (UAQCMD) and Canonical Monte-Carlo (CMC) methods to investigate the nucleation process. The UA-QCMD can calculate chemical reaction dynamics 107 times faster than conventional first principle molecular dynamics methods, while CMC can calculate equilibrium properties at various temperatures, pressures, and chemical compositions.