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Gasoline Compression Ignition (GCI) has been identified as a technology which could give both high efficiency and relatively low engine-out emissions. The introduction of any new vehicle technology requires widespread availability of appropriate fuels. It would be ideal therefore if GCI vehicles were able to operate using the standard grade of gasoline that is available at the pump. However, in spite of recent progress, operation at idle and low loads still remains a formidable challenge, given the relatively low autoignition reactivity of conventional gasoline at these conditions. One conceivable solution would be to use both diesel and gasoline, either in separate tanks or blended as a single fuel (“dieseline”). However, with this latter option, a major concern for dieseline would be whether a flammable mixture could exist in the vapour space in the fuel tank.