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Recent work has demonstrated the potential of gasoline-like fuels to reduce NOx and particulate emissions when used in Diesel engines. In this context, straight-run naphtha, a refinery stream directly derived from the atmospheric crude oil distillation process, has been identified as a highly valuable fuel. The current study is one step further toward naphtha-based fuel to power compression ignition engines. The potential of a cetane number 25 fuel (CN25), resulting from a blend of hydro-treated straight-run naphtha CN35 with unleaded non-oxygenated gasoline RON91 was assessed. For this purpose, investigations were conducted on multiple fronts, including experimental activities on an injection test bed, in an optically accessible vessel and in a single cylinder engine. CFD simulations were also developed to provide relevant explanations.