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The efficiency of spark ignition (SI) engines is usually limited by the occurrence of knock, which is linked to fuel octane number. If running the engine at its optimal efficiency requires a high octane number at high load, a lower octane number can be used at low load. Saudi Aramco, along with its long-term partner IFP Energies nouvelles, has been developing a synergistic fuel engine system where the engine is fed by fuel with an octane number adjusted in real time, on an as needed basis, while running at its optimal efficiency. Two major steps are identified to develop this “Octane on Demand” (OOD) concept: First, characterize the octane requirement needed to run the engine at its optimal efficiency over the entire map. Then, select the best dual fuel combination, including a base fuel and an octane booster to fit this concept.