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The transportation sector contributes significantly to emissions and air pollution globally. Emission models of modern vehicles are important tools to estimate the impact of technologies or controls on vehicle emission reductions, but developing a simple and high-fidelity model is challenging due to the variety of vehicle classes, driving conditions, driver behaviors, and other physical and operational constraints. Recent literature indicates that neural network-based models may be able to address these concerns due to their high computation speed and high-accuracy of predicted emissions. In this study, we seek to expand upon this initial research by utilizing several deep neural networks (DNN) architectures such as a recurrent neural network (RNN) and a convolutional neural network (CNN). These DNN algorithms are developed specific to the vehicle-out emissions prediction application, and a comprehensive assessment of their performances is done.