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Knocking is one phenomenon that can be cited as a factor impeding efforts to improve the efficiency of spark-ignition engines. With the aim of understanding knocking better, light emission spectroscopy was applied in this study to examine preflame reactions that can be observed prior to autoignition in the combustion reaction process of hydrocarbon fuels. Attention was focused on light emission behavior at wavelengths corresponding to those of formaldehyde (HCHO), Vaidya's hydrocarbon flame band (HCO) and the OH radical in a forced progression from normal combustion to a knocking state. Light emission behavior was measured simultaneously in the center and in the end zone of the combustion chamber when the engine was operated on two different test fuels. The test fuels used were n-heptane (0 RON) and a blended fuel (70 RON) consisting of n-heptane (0 RON) and iso-octane (100 RON).

With the aim of elucidating the mechanism generating knock, an examination was made of the preflame reaction behavior of end gas in the combustion chamber in the transition from normal combustion to abnormal combustion characterized by the occurrence of knocking. Simultaneous measurements were made in the same cycle of the light absorption and emission behavior of the OH (characteristic spectrum of 306.4 nm), CH (431.5 nm) and C2 (516.5 nm) radicals in the end-gas region using spectroscopic methods. The absorbance behavior of a blue flame prior to autoignition is believed to be an important factor in the mechanism causing knock.

The investigation regarding the plasma jet ignition was explored by using a combustion vessel. The first purpose is to elucidate the issuing duration and the penetration of hydrogen plasma jet. A temporal change of local electron temperature was measured along the central axis of plasma jet. A small characteristic length of igniter seems favorable with regard to the plasma jet penetration and the generation of high temperature, as compared with the case of the igniter that has the excessive cavity volume. The second purpose is to elucidate relationship between the characteristic length and the combustion enhancement effect, when the excessive volume of cavity and the excessive supplied electrical energy were used. The influence of the characteristic length on the plasma jet penetration and the combustion enhancement differs with the supplied energy. The combustion enhancement seems to be caused by the plasma jet in case of excessive supplied energy.

The purpose of this research was to obtain a better understanding of engine knocking phenomena. Measurements were made of the behavior of formaldehyde (HCHO), an important intermediate product of cool flame reactions, and of the HCO radical, characterized by distinctive light emission during blue flame reactions. The test engine was operated on a blended fuel (50 RON) of n-heptane and iso-octane. Simultaneous measurements were made of the behavior of HCHO and the OH radical using absorption spectroscopy and of the behavior of HCO and OH radicals using emission spectroscopy. Absorbance spectroscopic measurements revealed behavior thought to correspond to the passage of a cool flame and emission spectroscopic measurements showed behavior thought to correspond to the passage of a blue flame.

Emission intensity was measured at a wavelength of 395 2 nm (corresponding to the characteristic spectrum of the HCHO radical) and absorbance was measured at 306 4 nm (corresponding to that of the OH radical). The emission intensity and absorbance waveforms recorded during engine operation on n-heptane show behavior indicative of the passage and degeneracy of cool flame in the preflame reaction interval. As the combustion chamber wall temperature approached an overheated state in the transition from normal combustion to knocking operation different preflame reaction behavior was observed which is thought to correspond to the presence of a negative temperature coefficient region related to the ignition delay time.

The use of a higher compression ratio is desirable for improving the thermal efficiency and specific power of spark-ignition engines, but it gives rise to a problem of engine knock. In the present research, an investigation was made of the role of the preflame reaction region of a spark-ignition engine in the occurrence of autoignition. Emission spectroscopy was used to measure the behavior of formaldehyde (HCHO) in a cool flame. In addition, measure the behavior of the faint light attributed to the HCO radical in a blue flame with the concurrent measurement of the OH radical. The emission waveforms measurements obtained for HCHO when n-heptane (ORON) was used as the fuel, It is thought that these tendencies correspond to the passage and degeneracy of a cool flame. Further, the emission waveforms measured for the HCO radical when blended fuels (6ORON, 8ORON) were correspond to that of a blue flame.