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In-cylinder pre-processing (or recompression reaction) of direct-injected fuel during the negative valve overlap period of a retention-strategy HCCI engine is investigated for extension of the low-load limit of operation. Experimental studies of three variables (compression ratio, pilot injection timing, and pilot injection amount) were conducted in order to optimize the effects of recompression reaction by changing the sensible and chemical energy environment during recompression. The results from compression ratio variation show that there exist optimum values of equivalence ratio and extent of recompression reaction, which expand the low-load operating region. The pilot injection timing variation demonstrates good controllability of the extent of recompression reaction by effectively changing the in-cylinder residence time of the pilot-injected fuel.