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The detailed mechanisms by which oxygenated diesel fuels reduce engine-out soot emissions are not well understood. The literature contains conflicting results as to whether a fuel's overall oxygen content is the only important parameter in determining its soot-reduction potential, or if oxygenate molecular structure or other variables also play significant roles. To begin to resolve this controversy, experiments were conducted at a 1200-rpm, moderate-load operating condition using a modern-technology, 4-stroke, heavy-duty DI diesel engine with optical access. Images of broadband natural luminosity (i.e., light emission without spectral filtering) from the combustion chamber, coupled with heat-release and efficiency analyses, are presented for three test-fuels. One test-fuel (denoted GE80) was oxygenated with tri-propylene glycol methyl ether; the second (denoted BM88) was oxygenated with di-butyl maleate. The overall oxygen contents of these two fuels were matched at 26% by weight.

The accurate quantification and control of mixture stoichiometry is critical in many applications using new combustion strategies and fuels (e.g., homogeneous charge compression ignition, gasoline direct injection, and oxygenated fuels). The parameter typically used to quantify mixture stoichiometry (i.e., the proximity of a reactant mixture to its stoichiometric condition) is the equivalence ratio, ϕ. The traditional definition of ϕ is based on the relative amounts of fuel and oxidizer molecules in a mixture. This definition provides an accurate measure of mixture stoichiometry when the fuel molecule does not contain oxidizer elements and when the oxidizer molecule does not contain fuel elements. However, the traditional definition of ϕ leads to problems when the fuel molecule contains an oxidizer element, as is the case when an oxygenated fuel is used, or once reactions have started and the fuel has begun to oxidize.

The influence of nitrogen dilution and charge-gas temperature on in-cylinder combustion processes and engine-out NOx and smoke emissions was investigated in an optically accessible heavy-duty DI diesel engine using a high-cetane-number, oxygenated fuel. Engine-out measurements of NOx and smoke emissions and in-cylinder images of natural luminosity were obtained for charge-gas oxygen concentrations from 9% to 21% and TDC charge-gas temperatures of 680 and 880 K. Charge-gas temperature was found to have a significant influence on engine-out NOx emissions, but NOx emissions levels less than 0.2 g/ihp-hr were achieved at both the 680 and 880 K charge-gas temperatures within the investigated range of oxygen concentrations. An indicated engine-out NOx emissions level of 0.09 g/ihp-hr at 18 bar IMEP was achieved using charge-gas dilution and 3.0 bar intake boost pressure.