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Precipitation chemistry measurements have been made at many California locations, with recorded extreme pH values as low as 2.89 from Pasadena and 3.5 from geologically sensitive Sequoia National Park. However, in northern areas of the state experiencing good air quality, very little acid deposition occurs. California's acid precipitation is apparently locally produced, since there are no major pollution source regions upwind of the state. This is attributable to the extremely rapid rates observed for conversion of NOx to nitric acid and SO2 to sulfuric acid in the atmosphere. Recent monitoring data illustrate extreme variations in precipitation chemistry from adjacent sites and even at the same location from one year to the next. Enrichment factor calculations show that in contrast with data from other locations in the world, nitric acid dominates over sulfuric acid in California's rainfall in many locations.

This paper summarizes current work in the Environmental Science & Health Effects (ES&HE) Program being sponsored by DOE's Office of Heavy Vehicle Technologies (OHVT) through the National Renewable Energy Laboratory (NREL). The program is regulatory-driven, and focuses on ozone, airborne particles, visibility and regional haze, air toxics, and health effects of air pollutants. The goal of the ES&HE Program is to understand atmospheric impacts and potential health effects that may be caused by the use of petroleum-based and alternative transportation fuels. Each project in the program is designed to address policy-relevant objectives. Studies in the ES&HE Program have four areas of focus: improving technology for emissions measurements; vehicle emissions measurements, emission inventory development/improvement; and ambient impacts, including health effects.

To help guide heavy vehicle engine, fuel, and exhaust after-treatment technology development, the U.S. Department of Energy and the Lovelace Respiratory Research Institute are conducting research not addressed elsewhere on aspects of the toxicity of particulate engine emissions. Advances in these technologies that reduce diesel particulate mass emissions may result in changes in particle composition, and there is concern that the number of ultrafine (<0.1 micron) particles may increase. All present epidemiological and laboratory data on the toxicity of diesel emissions were derived from emissions of older-technology engines. New, short-term toxicity data are needed to make health-based choices among diesel technologies and to compare the toxicity of diesel emissions to those of other engine technologies.