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This paper presents experimental results regarding a new approach to smart radiator devices (SRD) employing a smart, integrated thin-film structure based on V1-x-yMxNyOn that can be applied to existing thermal blankets such as Kapton or to thermal radiators such as Al. The smart coating facilitates thermal control by dynamically modifying the thermo-optic characteristics of the underlying substrate in response to the ambient temperature and/or a control voltage. This methodology has significant advantages over competitive technologies in terms of weight, cost, structural simplicity, and integration with the space structure. The effective emissivity of the film/substrate structure can be reduced dynamically by changing the behavior of the smart coating from insulator to metallic. High quality VO2 films have been prepared using a hybrid reactive laser ablation technique.