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Autoignition correlations are widely used to predict knock in internal combustion engines as opposed to detailed kinetics mechanisms involving hundreds of reactions due to computational cost. Several autoignition correlations exist in the literature for different fuels, and their functional form depends on the operating parameters like fuel type and temperature range, among other things. In the literature different types of correlations are proposed for gasoline fuel, but to the best of the authors’ knowledge none of these correlations can be used for gasoline-ethanol blends with varying levels of ethanol percentage and a wide range of equivalence ratios and temperatures. In this paper, a new empirical correlation is developed to predict the autoignition of gasoline-ethanol blends over a wide range of temperatures including Negative Temperature Coefficient (NTC) region.