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In order to better understand in-flame diesel soot oxidation processes, soot particles at the oxidation-dominant periphery of diesel spray flame were sampled by a newly developed “suck” type soot sampler employing a high-speed solenoid valve and their morphology and nanostructure were observed via high-resolution transmission electron microscopy (HR-TEM). A single-shot diesel spray flame for the soot sampling experiment was achieved in a constant-volume vessel under a diesel-like condition. The sampler instantaneously sucks out a small portion of soot laden gases from the flame. A TEM grid holds inside the flow passage close to its entrance is immediately exposed to the gas flow induced by the suction at the upstream of the solenoid valve, so that the quick thermophoretic soot deposition onto the grid surface can effectively freeze morphology variation of soot particles during the sampling processes.

The enhancement of vortex development, fuel-air mixing and heat release in diesel spray flame by inversed-delta injection rate shaping, having been predicted via LES simulation with detailed chemical kinetics, is experimentally confirmed for the first time. Newly developed 3-injector TAIZAC (TAndem Injector Zapping ACtivation) injector realizing aggressive inversed-delta injection rate shaping was used for single-shot combustion experiments in a constant volume combustion vessel. Simultaneous high-speed (120,000fps) and high-resolution (1,280 x 704 pixels) laser schlieren and UV OH* chemiluminescence imaging combined with subsequent Flame Imaging Velocimetry (FIV) analysis was employed to elucidate the correlation between vortex development and enhanced heat release.

Measurements of Excitation-Emission Matrix (EEM) of shock-heated vapors of polycyclic aromatic hydrocarbons (PAHs) at high temperature (750-1500K) and high pressure (0.3-1.3MPa) conditions were conducted using a multi-wavelength excitation laser in order to demonstrate the potential of the single-measurement EEM fluorometry for investigation of soot precursors. Argon-diluted vapors of naphthalene and pyrene, as PAH model compounds, were heated in an optically accessible shock tube. The PAH vapors were excited by a coherent multi-wavelength “rainbow” laser light generated by converting the 4th harmonic (266nm) of a pulsed Nd:YAG laser using a Raman cell frequency converter filled with high-pressure (2MPa) methane-hydrogen mixture.

In order to investigate the soot formation process in a diesel spray flame, simultaneous imaging of soot precursor and soot particles in a transient spray flame achieved in a rapid compression machine was conducted by laser-induced fluorescence (LIF) and by laser-induced incandescence (LII) techniques. The 3rd harmonic (355nm) and the fundamental (1064nm) laser pulses from an Nd:YAG laser, between which a delay of 44ns was imposed by 13.3m of optical path difference, were used to excite LIF from soot precursor and LII from soot particles in the spray flame. The LIF and the LII were separately imaged by two image-intensified CCD cameras with identical detection wavelength of 400nm and bandwidth of 80nm. The LIF from soot precursor was mainly located in the central region of the spray flame between 40 and 55mm (270 to 370 times nozzle orifice diameter d0) from the nozzle orifice. The LII from soot particles was observed to surround the soot precursor LIF region and to extend downstream.