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A premixed charge compression ignition methanol engine targeting a drastic decrease in NOx emissions and a brake specific energy consumption equivalent to that of a DI diesel engine has been developed (1). The problems of this combustion system are that the brake thermal efficiency decreases, and CO and THC emissions increase due to a deterioration of high load combustion. The purpose of this study is to improve the high load combustion of a premixed charge compression ignition methanol engine using a flash boiling fuel injection technique. The results of this study have shown that the premixed charge compression ignition methanol combustion system using a flash boiling fuel injection technique increases the brake thermal efficiency, decreases CO and THC emissions, while maintaining low NOx emissions in the high load region.