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The three-way-catalyst (TWC) is an essential part of the exhaust aftertreatment system in spark-ignited powertrains, converting nearly all toxic emissions to harmless gasses. The TWC’s conversion efficiency is significantly temperature-dependent, and cold-starts can be the dominating source of emissions for vehicles with frequent start/stops (e.g. hybrid vehicles). In this paper we develop a thermal TWC model and calibrate it with experimental data. Due to the few number of state variables the model is well suited for fast offline simulation as well as subsequent on-line control, for instance using non-linear state-feedback or explicit MPC. Using the model could allow an on-line controller to more optimally adjust the engine ignition timing, the power in an electric catalyst pre-heater, and/or the power split ratio in a hybrid vehicle when the catalyst is not completely hot.

In engine research and development there are often different engine parameters that produce similar effects on the end-point results. When calibrating modern engines, a huge number of parameters needs to be set, which also includes compensation parameters for model imperfections. In this context, simpler, more robust, and physically based models should be beneficial both for calibration work load and powertrain performance. In this study, we present an experimental methodology that uses intermediate (“intrinsic”) variables instead of engine parameters. By using simple thermodynamic models, the engine parameters EGR, IVC, and PBoost could be translated into oxygen concentration, temperature and gas density at the start of injection. The reason for this transformation of data is to “move” the Design of Experiment (DoE) closer to the situation of interest (i.e. the combustion) and to be able to construct simpler and more physically based models.