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Molecular decomposition is a key chemical process in combustion systems. Particularly, the spatio-temporal information related to a fuel’s molecular breakdown is of high-importance regarding the development of combustion models and more specifically about chemical kinetic mechanisms. Most experiments rely on a variety of ultraviolet or infrared techniques to monitor the fuel breakdown process in 0-D type experiments such as those performed in shock-tubes or rapid compression machines. While the information provided by these experiments is necessary to develop and adjust kinetic mechanisms, they fail to provide the necessary data for applied combustion models to be predictive regarding the fuel’s molecular breakdown. In this work, we investigated the molecular decomposition of a fuel by applying high-speed planar laser Rayleigh scattering (PLRS).

The 4th Workshop of the Engine Combustion Network (ECN) was held September 5-6, 2015 in Kyoto, Japan. This manuscript presents a summary of the progress in experiments and modeling among ECN contributors leading to a better understanding of soot formation under the ECN “Spray A” configuration and some parametric variants. Relevant published and unpublished work from prior ECN workshops is reviewed. Experiments measuring soot particle size and morphology, soot volume fraction (fv), and transient soot mass have been conducted at various international institutions providing target data for improvements to computational models. Multiple modeling contributions using both the Reynolds Averaged Navier-Stokes (RANS) Equations approach and the Large-Eddy Simulation (LES) approach have been submitted. Among these, various chemical mechanisms, soot models, and turbulence-chemistry interaction (TCI) methodologies have been considered.

This work investigates the injection processes of an eight-hole direct-injection gasoline injector from the Engine Combustion Network (ECN) effort on gasoline sprays (Spray G). Experiments are performed at identical operating conditions by multiple institutions using standardized procedures to provide high-quality target datasets for CFD spray modeling improvement. The initial conditions set by the ECN gasoline spray community (Spray G: Ambient temperature: 573 K, ambient density: 3.5 kg/m3 (∼6 bar), fuel: iso-octane, and injection pressure: 200 bar) are examined along with additional conditions to extend the dataset covering a broader operating range. Two institutes evaluated the liquid and vapor penetration characteristics of a particular 8-hole, 80° full-angle, Spray G injector (injector #28) using Mie scattering (liquid) and schlieren (vapor).

Multi-hole diesel fuel injectors have shown significant transients in spreading angle during injections, different than past fundamental research using single-hole injectors. We investigated the effect of a this transient spreading angle on combustion parameters such as ignition delay and lift-off length by comparing a three-hole nozzle (Spray B) and single-hole nozzle (Spray A) with holes of the same size and shape as targets for the Engine Combustion Network (ECN). With the temperature distribution for a target plume of Spray B characterized extensively in a constant-volume combustion chamber, the ignition delay and lift-off length were measured and compared. Results show that the lift-off length of Spray B increases and grows by approximately 1.5 mm after the initial stages of ignition, in an opposite trend compared to Spray A where the lift-off length decreases with time.

We investigate the mixing, penetration, and ignition characteristics of high-pressure n-dodecane sprays having a split injection schedule (0.5/0.5 dwell/0.5 ms) in a pre-burn combustion vessel at ambient temperatures of 750 K, 800 K and 900 K. High-speed imaging techniques provide a time-resolved measure of vapor penetration and the timing and progression of the first- and second-stage ignition events. Simultaneous single-shot planar laser-induced fluorescence (PLIF) imaging identifies the timing and location where formaldehyde (CH2O) is produced from first-stage ignition and consumed following second-stage ignition. At the 900-K condition, the second injection penetrates into high-temperature combustion products remaining in the near-nozzle region from the first injection. Consequently, the ignition delay for the second injection is shorter than that of the first injection (by a factor of two) and the second injection ignites at a more upstream location near the liquid length.

The mixing field of sprays injected into high temperature and pressure environments has been observed to be tightly connected to spreading angle, therefore linking vaporization and combustion processes to the angular dispersion of the spray. Visualization of the Engine Combustion Network three-hole, Spray B diesel injector shows substantial variation in near-field spreading angle with respect to time compared to past measurements of the single-hole, Spray A injector. The source of these variations originating inside the nozzle, and the implications on mixing, evaporation, and combustion of the diesel plume, need to be understood. In this study, we characterize the ECN-target plume for a Spray B injector (Serial # 211201), which already benefits from extensive and detailed internal measurements of nozzle geometry and needle movement, while comparing to the single-hole Spray A with the same type of detailed geometry and understanding.

The Leaner Lifted-Flame Combustion (LLFC) strategy offers a possible alternative to low temperature combustion or other globally lean, premixed operation strategies to reduce soot directly in the flame, while maintaining mixing-controlled combustion. Adjustments to fuel properties, especially fuel oxygenation, have been reported to have potentially beneficial effects for LLFC applications. Six fuels were selected or blended based on cetane number, oxygen content, molecular structure, and the presence of an aromatic hydrocarbon. The experiments compared different fuel blends made of n-hexadecane, n-dodecane, methyl decanoate, tri-propylene glycol monomethyl ether (TPGME), as well as m-xylene. Several optical diagnostics have been used simultaneously to monitor the ignition, combustion and soot formation/oxidation processes from spray flames in a constant-volume combustion vessel.

A full understanding and characterization of the near-field of diesel sprays is daunting because the dense spray region inhibits most diagnostics. While x-ray diagnostics permit quantification of fuel mass along a line of sight, most laboratories necessarily use simple lighting to characterize the spray spreading angle, using it as an input for CFD modeling, for example. Questions arise as to what is meant by the “boundary” of the spray since liquid fuel concentration is not easily quantified in optical imaging. In this study we seek to establish a relationship between spray boundary obtained via optical diffused backlighting and the fuel concentration derived from tomographic reconstruction of x-ray radiography. Measurements are repeated in different facilities at the same specified operating conditions on the “Spray A” fuel injector of the Engine Combustion Network, which has a nozzle diameter of 90 μm.

Transients in the rate of injection (ROI) with respect to time are ever-present in direct-injection engines, even with common-rail fueling. The shape of the injection ramp-up and ramp-down affects spray penetration and mixing, particularly with multiple-injection schedules currently in practice. Ultimately, the accuracy of CFD model predictions used to optimize the combustion process depends upon the accuracy of the ROI utilized as fuel input boundary conditions. But experimental difficulties in the measurement of ROI, as well as real-world affects that change the ROI from the bench to the engine, add uncertainty that may be mistaken for weaknesses in spray modeling instead of errors in boundary conditions. In this work we use detailed, time-resolved measurements of penetration at the Spray A conditions of the Engine Combustion Network to rigorously guide the necessary ROI shape required to match penetration in jet models that allow variable rate of injection.