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This paper describes a numerical analysis method for predicting the brake squeal using the Substructure Synthesis Method. This method is more accurate than the classical method based on the mass-spring system, and simpler than the analysis of all the brake system by FEM. The squeal studied here is focused the one occurring in the low frequency range and its mechanism is due the structural instability of the brake assembly. First, some experiments were carried out in order to grasp the brake squeal phenomenon. These experiments made clear the following items. (1) The low frequency brake squeal occurred at 850Hz. (2) The vibration mode shape had 5 nodes fixed in a space. (3) The brake squeal became maximum at 0.3 - 0.5 (MPa) liquid pressure under the constant temperature condition. (4) The higher the temperature of the pad was, the stronger the brake squeal was under the constant liquid pressure condition.