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The dilution of the cylinder charge using excess air enables both an increase in the net indicated efficiency and a decrease in the engine-out emissions of nitrogen oxides. The maximum excess air dilution capability in a spark-ignition engine depends on both the ignition of the charge and the flame propagation. These two aspects can be influenced by the fuel properties, which draw attention to the laminar burning velocity of alternative fuels to extend the lean limit. Cyclopentanone and anisole show promising values regarding the laminar burning velocity. However, there is a lack of engine investigations using these two fuels. To this end, both fuels were assessed in an engine application using experimental and numerical investigations. Cyclopentanone and anisole were investigated as neat components and as mixtures with conventional gasoline fuel, resulting in seven investigated fuels.