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A growing interest towards heavy-duty engines powered with NG, dictated by stringent regulations in terms of emissions, has made it essential to study a specific Three-Way Catalyst (TWC). Oxygen storage phenomena characterize the catalytic converter efficiency under real world driving operating conditions and, consequently, during strong dynamics in Air-to-Fuel ratio (AFR). A numerical “quasi-steady” model has been set-up to simulate the chemical process inside the reactor. A dedicated experimental campaign has been performed in order to evaluate the catalyst response to a defined λ variation, thus providing the data necessary for the numerical model validation. In fact, goal of the present research activity was to investigate the effect of very fast composition transitions of the engine exhaust typical of the mentioned driving conditions (including fuel cutoffs etc.) on the catalyst performance and on related emissions.

Effects of n-butanol on the combustion process in a direct injection spark ignition engine were investigated through flame visualization and spectroscopy. An optically accessible engine was equipped for the trials with a commercial cylinder head and wall guided injection system. Injection pressure (100 bar) and engine speed (2000 rpm) were fixed while injection timing and duration were changed to realise stoichiometric and lean fuelling in homogenous charge conditions. Specifically, UV-visible digital imaging was applied in order to study the flame front inception and propagation with particular interest in the early combustion stages. UV-visible natural emission spectroscopy was applied to investigate the formation and the evolution of the main chemical compounds characterizing the spark ignition and combustion processes. Detailed image processing allowed to correlate the morphology and the local flame front curvature with thermodynamic data.