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Although methane number is widely used to predict knocking occurrence and its intensity, it does not determine a fuel composition uniquely, that means, the knocking intensity by the different composition fuel must show difference even if the same methane number fuels are employed. To establish a novel index, the knocking intensity and the autoignitive propagation velocity, as consequence of spontaneous ignition process, are investigated both experimentally and numerically by using the different composition gaseous fuels with same methane number. Methane/ethane/air and methane/n-butane/air mixtures with the same methane number of 70 and the equivalence ratio of 0.5 were employed. They are rapidly compressed and ignited spontaneously by a Rapid Compression Machine. Ignition delay times, autoignitive propagation velocities, and knocking intensity were measured by acquired pressure histories and high-speed imaging.