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Adaptation of predictive combustion models for their use in in-cycle closed-loop combustion control of a multi-cylinder engine is studied in this article. Closed-loop combustion control can adjust the operation of the engine closer to the optimal point despite production tolerances, component variations, normal disturbances, ageing or fuel type. In the fastest loop, in-cycle closed-loop combustion control was proved to reduce normal variations around the operational point to increase the efficiency. However, these algorithms require highly accurate predictive models, whilst having low complexity for their implementation. Three models were used to exemplify the proposed adaptation methods: the pilot injection’s ignition delay, the pilot burned mass, and the main injection’s ignition delay. Different approaches for the adaptation of the models are studied to obtain the demanded accuracy under the implementation constraints.