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Strict NOx and soot emission regulations for Diesel engines have created an interest in low-temperature partially-homogeneous combustion regimes in both the US and Europe. One strategy, Homogeneous-Charge Late-Injection (HCLI) combustion utilizes 55% or more cooled external Exhaust Gas Recirculation (EGR) with a single Direct Injection strategy to control ignition timing. These engines are operated at low temperatures to ensure near zero NOx emissions, implying that fuel in the thermal boundary layers will not reach sufficient temperature to fully oxidize, resulting in Unburnt Hydrocarbon (UHC) and CO emissions. Of particular interest to HCLI engines are the UHC's that are not fully oxidized by the Diesel Oxidation Catalyst (DOC). Experimental measurements reveal that at average equivalence ratios greater than 0.8, methane is the single largest tailpipe-out UHC emission.